Abstract
We report neutron scattering and ac susceptibility measurements on the pyrochlore Yb2Sn2O7. The appearance of magnetic diffuse scattering, low-energy spin excitations, and a nearly temperature-independent relaxation time are signatures that the system enters a short-range-ordered regime with quantum dynamics beneath 2 K. ac susceptibility data further suggest that Yb2Sn2O7 enters a long-range magnetically ordered state below 0.11 K. These results suggest that Yb2Sn2O7 is a ferromagnet with persistent spin dynamics down to 0.05 K. Referencing the phase diagram for Yb pyrochlores, Yb2Sn2O7 is approaching a quantum phase transition near the ferromagnetic ordered critical point.
Original language | English |
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Article number | 134408 |
Journal | Physical Review B - Condensed Matter and Materials Physics |
Volume | 87 |
Issue number | 13 |
DOIs | |
State | Published - Apr 10 2013 |
Externally published | Yes |