Weak localization competes with the quantum oscillations in a natural electronic superlattice: The case of Na1.5(PO2)4(WO3)20

Kamil K. Kolincio, Olivier Pérez, Enric Canadell, Pere Alemany, Elen Duverger-Nédellec, Arianna Minelli, Alexei Bosak, Alain Pautrat

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Abstract

We report an investigation of the combined structural and electronic properties of the bronze Na1.5(PO2)4(WO3)20. Its low-dimensional structure and possible large reconstruction of the Fermi surface due to charge density wave instability make this bulk material a natural superlattice with a reduced number of carriers and Fermi energy. Signatures of multilayered two-dimensional (2D) electron weak localization are consequently reported, with an enhanced influence of quantum oscillations. A crossover between these two antagonistic entities, previously observed only in genuine low-dimensional materials and devices, is shown to occur in a bulk crystal due to its hidden 2D nature.

Original languageEnglish
Article number161117
JournalPhysical Review B
Volume101
Issue number16
DOIs
StatePublished - Apr 15 2020
Externally publishedYes

Funding

A.P. would like to thank Thierry Klein and Andrea Gauzzi for valuable remarks on the competition between weak localization and quantum oscillation conditions which motivated our analysis. Financial support by the ANR Projects No. ANR-18-CE92-0014 and No. ANR-11-BS04-0004 is gratefully acknowledged. Work in Spain was supported by MICIU (PGC2018-096955-B-C44 and PGC2018-093863-B-C22), MINECO through the Severo Ochoa (SEV-2015-0496) and Maria de Maeztu (MDM-2017-0767) Programs, and the Generalitat de Catalunya (2017SGR1506 and 2017SGR1289). E.D.-N. was supported by the project NanoCent-Nanomaterials center for advanced applications, Project No. CZ.02.1.01/0.0/0.0/15_003/0000485, financed by the ERDF.

FundersFunder number
MICIUPGC2018-096955-B-C44, PGC2018-093863-B-C22
Maria de MaeztuMDM-2017-0767
Generalitat de CatalunyaCZ.02.1.01/0.0/0.0/15_003/0000485, 2017SGR1506, 2017SGR1289
Ministerio de Economía y CompetitividadSEV-2015-0496
European Regional Development Fund

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