Visualizing the interplay of Dirac mass gap and magnetism at nanoscale in intrinsic magnetic topological insulators

Mengke Liu, Chao Lei, Hyunsue Kim, Yanxing Li, Lisa Frammolino, Jiaqiang Yan, Allan H. Macdonald, Chih Kang Shih

Research output: Contribution to journalArticlepeer-review

19 Scopus citations

Abstract

In intrinsic magnetic topological insulators, Dirac surface-state gaps are prerequisites for quantum anomalous Hall and axion insulating states. Unambiguous experimental identification of these gaps has proved to be a challenge, however. Here, we use molecular beam epitaxy to grow intrinsic MnBi2Te4 thin films. Using scanning tunneling microscopy/spectroscopy, we directly visualize the Dirac mass gap and its disappearance below and above the magnetic order temperature. We further reveal the interplay of Dirac mass gaps and local magnetic defects. We find that, in high defect regions, the Dirac mass gap collapses. Ab initio and coupled Dirac cone model calculations provide insight into the microscopic origin of the correlation between defect density and spatial gap variations. This work provides unambiguous identification of the Dirac mass gap in MnBi2Te4 and, by revealing the microscopic origin of its gap variation, establishes a material design principle for realizing exotic states in intrinsic magnetic topological insulators.

Original languageEnglish
Article numbere2207681119
JournalProceedings of the National Academy of Sciences of the United States of America
Volume119
Issue number42
DOIs
StatePublished - Oct 18 2022

Keywords

  • Dirac mass gap
  • STM/STS
  • magnetic topological insulator
  • topological phase transition

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