Unleashing the Potential of NASICON Materials for Solid-State Batteries

Anand Parejiya; Marm Dixit; Rachid Essehli; Ruhul Amin; Ilias Belharouak

doi:10.1007/s11837-023-06291-7

Unleashing the Potential of NASICON Materials for Solid-State Batteries

Anand Parejiya, Marm Dixit, Rachid Essehli, Ruhul Amin, Ilias Belharouak

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

Solid-state batteries (SSBs) represent a transformative technology with the potential to redefine energy storage in various applications, including portable electronics, electric vehicles, and renewable energy systems. However, the intricate interplay of materials and interfaces within SSBs poses significant challenges in realizing their full potential. In this perspective, we highlight the potential of integration of NASICON (Sodium Superionic Conductor) materials into SSB architectures to address compatibility issues and enhance overall performance. We also showcase that, by employing machine learning techniques and a data-driven approach, structure-function relationships governing NASICON materials’ ionic conductivity can be perceived. This eliminates the need for computationally intensive first-principles calculations and offers insights into the mechanism of improving ion transport. Our findings highlight the promise of NASICON-type materials in overcoming chemical, mechanical, and electrochemical disparities at interfaces and interphases, offering a promising path forward for the development of high-performance SSBs.

Original language	English
Pages (from-to)	1088-1093
Number of pages	6
Journal	JOM
Volume	76
Issue number	3
DOIs	https://doi.org/10.1007/s11837-023-06291-7
State	Published - Mar 2024

Funding

This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan ( http://energy.gov/downloads/doe-public-access-plan ). This research at Oak Ridge National Laboratory, managed by UT Battelle, LLC, for the US Department of Energy (DOE) under contract DE-AC05-00OR22725, was sponsored by Laboratory Directed Research and Development (LDRD) Program at Oak Ridge National Laboratory, and the Office of Energy Efficiency and Renewable Energy (EERE) Vehicle Technologies Office (VTO) Applied Battery Research subprogram. Marm Dixit is supported by the Alvin M. Weinberg Fellowship at Oak Ridge National Laboratory.

Funders	Funder number
U.S. Department of Energy	DE-AC05-00OR22725
Office of Energy Efficiency and Renewable Energy
Oak Ridge National Laboratory
Laboratory Directed Research and Development
UT-Battelle

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1007/s11837-023-06291-7

Cite this

@article{30a691f4876c468ca1c15254d56f3e8b,

title = "Unleashing the Potential of NASICON Materials for Solid-State Batteries",

abstract = "Solid-state batteries (SSBs) represent a transformative technology with the potential to redefine energy storage in various applications, including portable electronics, electric vehicles, and renewable energy systems. However, the intricate interplay of materials and interfaces within SSBs poses significant challenges in realizing their full potential. In this perspective, we highlight the potential of integration of NASICON (Sodium Superionic Conductor) materials into SSB architectures to address compatibility issues and enhance overall performance. We also showcase that, by employing machine learning techniques and a data-driven approach, structure-function relationships governing NASICON materials{\textquoteright} ionic conductivity can be perceived. This eliminates the need for computationally intensive first-principles calculations and offers insights into the mechanism of improving ion transport. Our findings highlight the promise of NASICON-type materials in overcoming chemical, mechanical, and electrochemical disparities at interfaces and interphases, offering a promising path forward for the development of high-performance SSBs.",

author = "Anand Parejiya and Marm Dixit and Rachid Essehli and Ruhul Amin and Ilias Belharouak",

note = "Publisher Copyright: {\textcopyright} The Minerals, Metals & Materials Society 2023.",

year = "2024",

month = mar,

doi = "10.1007/s11837-023-06291-7",

language = "English",

volume = "76",

pages = "1088--1093",

journal = "JOM",

issn = "1047-4838",

publisher = "Springer",

number = "3",

}

TY - JOUR

T1 - Unleashing the Potential of NASICON Materials for Solid-State Batteries

AU - Parejiya, Anand

AU - Dixit, Marm

AU - Essehli, Rachid

AU - Amin, Ruhul

AU - Belharouak, Ilias

PY - 2024/3

Y1 - 2024/3

N2 - Solid-state batteries (SSBs) represent a transformative technology with the potential to redefine energy storage in various applications, including portable electronics, electric vehicles, and renewable energy systems. However, the intricate interplay of materials and interfaces within SSBs poses significant challenges in realizing their full potential. In this perspective, we highlight the potential of integration of NASICON (Sodium Superionic Conductor) materials into SSB architectures to address compatibility issues and enhance overall performance. We also showcase that, by employing machine learning techniques and a data-driven approach, structure-function relationships governing NASICON materials’ ionic conductivity can be perceived. This eliminates the need for computationally intensive first-principles calculations and offers insights into the mechanism of improving ion transport. Our findings highlight the promise of NASICON-type materials in overcoming chemical, mechanical, and electrochemical disparities at interfaces and interphases, offering a promising path forward for the development of high-performance SSBs.

AB - Solid-state batteries (SSBs) represent a transformative technology with the potential to redefine energy storage in various applications, including portable electronics, electric vehicles, and renewable energy systems. However, the intricate interplay of materials and interfaces within SSBs poses significant challenges in realizing their full potential. In this perspective, we highlight the potential of integration of NASICON (Sodium Superionic Conductor) materials into SSB architectures to address compatibility issues and enhance overall performance. We also showcase that, by employing machine learning techniques and a data-driven approach, structure-function relationships governing NASICON materials’ ionic conductivity can be perceived. This eliminates the need for computationally intensive first-principles calculations and offers insights into the mechanism of improving ion transport. Our findings highlight the promise of NASICON-type materials in overcoming chemical, mechanical, and electrochemical disparities at interfaces and interphases, offering a promising path forward for the development of high-performance SSBs.

UR - http://www.scopus.com/inward/record.url?scp=85179359582&partnerID=8YFLogxK

U2 - 10.1007/s11837-023-06291-7

DO - 10.1007/s11837-023-06291-7

M3 - Article

AN - SCOPUS:85179359582

SN - 1047-4838

VL - 76

SP - 1088

EP - 1093

JO - JOM

JF - JOM

IS - 3

ER -

Unleashing the Potential of NASICON Materials for Solid-State Batteries

Abstract

Funding

UN SDGs

Access to Document

Other files and links

Fingerprint

Cite this