Unidirectional coherent quasiparticles in the high-temperature rotational symmetry broken phase of AV3Sb5 kagome superconductors

Hong Li, He Zhao, Brenden R. Ortiz, Yuzki Oey, Ziqiang Wang, Stephen D. Wilson, Ilija Zeljkovic

Research output: Contribution to journalArticlepeer-review

33 Scopus citations

Abstract

Kagome metals AV3Sb51 (where the A can stand for K, Cs or Rb) display a rich phase diagram of correlated electron states, including superconductivity2–4 and density waves5–7. Within this landscape, recent experiments have revealed signs of a transition below approximately 35 K attributed to an electronic nematic phase that spontaneously breaks the rotational symmetry of the lattice8. Here we show that the rotational symmetry breaking initiates universally at a high temperature in these materials, towards the 2 × 2 charge density wave transition temperature. We do this via spectroscopic-imaging scanning tunnelling microscopy and study the atomic-scale signatures of the electronic symmetry breaking across several materials in the AV3Sb5 family: CsV3Sb5, KV3Sb5 and Sn-doped CsV3Sb5. Below a substantially lower temperature of about 30 K, we measure the quantum interference of quasiparticles, a key signature for the formation of a coherent electronic state. These quasiparticles display a pronounced unidirectional feature in reciprocal space that strengthens as the superconducting state is approached. Our experiments reveal that high-temperature rotation symmetry breaking and the charge ordering states are separated from the superconducting ground state by an intermediate-temperature regime with coherent unidirectional quasiparticles. This picture is phenomenologically different compared to that in high-temperature superconductors, shedding light on the complex nature of rotation symmetry breaking in AV3Sb5 kagome superconductors.

Original languageEnglish
Pages (from-to)637-643
Number of pages7
JournalNature Physics
Volume19
Issue number5
DOIs
StatePublished - May 2023
Externally publishedYes

Funding

We thank L. Balents, R. Fernandes, L. Wu and R. Comin for their insightful conversations. I.Z. gratefully acknowledges the support from grant no. NSF-DMR 2216080. S.D.W. and B.R.O. acknowledge support from the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under award no. DMR-1906325. Z.W. acknowledges the support of the US Department of Energy, Basic Energy Sciences grant no. DE-FG02-99ER45747 and the Cottrell SEED award no. 27856 from the Research Corporation for Science Advancement.

FundersFunder number
Cottrell SEED27856
UC Santa Barbara NSFDMR-1906325
U.S. Department of Energy
Research Corporation for Science Advancement
Basic Energy SciencesDE-FG02-99ER45747

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