Abstract
Kagome metals AV3Sb51 (where the A can stand for K, Cs or Rb) display a rich phase diagram of correlated electron states, including superconductivity2–4 and density waves5–7. Within this landscape, recent experiments have revealed signs of a transition below approximately 35 K attributed to an electronic nematic phase that spontaneously breaks the rotational symmetry of the lattice8. Here we show that the rotational symmetry breaking initiates universally at a high temperature in these materials, towards the 2 × 2 charge density wave transition temperature. We do this via spectroscopic-imaging scanning tunnelling microscopy and study the atomic-scale signatures of the electronic symmetry breaking across several materials in the AV3Sb5 family: CsV3Sb5, KV3Sb5 and Sn-doped CsV3Sb5. Below a substantially lower temperature of about 30 K, we measure the quantum interference of quasiparticles, a key signature for the formation of a coherent electronic state. These quasiparticles display a pronounced unidirectional feature in reciprocal space that strengthens as the superconducting state is approached. Our experiments reveal that high-temperature rotation symmetry breaking and the charge ordering states are separated from the superconducting ground state by an intermediate-temperature regime with coherent unidirectional quasiparticles. This picture is phenomenologically different compared to that in high-temperature superconductors, shedding light on the complex nature of rotation symmetry breaking in AV3Sb5 kagome superconductors.
Original language | English |
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Pages (from-to) | 637-643 |
Number of pages | 7 |
Journal | Nature Physics |
Volume | 19 |
Issue number | 5 |
DOIs | |
State | Published - May 2023 |
Externally published | Yes |
Funding
We thank L. Balents, R. Fernandes, L. Wu and R. Comin for their insightful conversations. I.Z. gratefully acknowledges the support from grant no. NSF-DMR 2216080. S.D.W. and B.R.O. acknowledge support from the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under award no. DMR-1906325. Z.W. acknowledges the support of the US Department of Energy, Basic Energy Sciences grant no. DE-FG02-99ER45747 and the Cottrell SEED award no. 27856 from the Research Corporation for Science Advancement.
Funders | Funder number |
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Cottrell SEED | 27856 |
UC Santa Barbara NSF | DMR-1906325 |
U.S. Department of Energy | |
Research Corporation for Science Advancement | |
Basic Energy Sciences | DE-FG02-99ER45747 |