Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology

Haoran Yu; Andrea Baricci; Justin Roller; Yang Wang; Andrea Casalegno; William E. Mustain; Radenka Maric

doi:10.1149/06917.0487ecst

Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology

Haoran Yu, Andrea Baricci, Justin Roller, Yang Wang, Andrea Casalegno, William E. Mustain, Radenka Maric

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

13 Scopus citations

Abstract

Reactive spray deposition technology (RSDT) is a cost-effective method for producing high performance proton exchange membrane fuel cell (PEMFC) membrane electrode assemblies (MEAs). In this study, we used the RSDT process to deposit catalyst-coated membrane (CCM) with Pt supported on Ketjen Black (KB), multi-wall carbon nanotube (MWCNT) and reducedgraphene oxide (rGO) with ultra-low Pt loading in order to elucidate the influence of the support and Pt dispersion on the catalyst perfromance. The electrochemically active surface area (ECSA), activity for oxygen reduction reaction (ORR) and PEMFC performance are investigated and compared.

Original language	English
Title of host publication	Polymer Electrolyte Fuel Cells 15, PEFC 15
Editors	H. A. Gasteiger, A. Z. Weber, V. K. Ramani, T. F. Fuller, R. A. Mantz, H. Uchida, F. N. Buchi, M. Edmundson, C. Coutanceau, J. M. Fenton, S. Mitsushima, T. J. Schmidt, K. Shinohara, K. Swider-Lyons, D. J. Jones, B. S. Pivovar, K. E. Ayers, K. A. Perry, S. R. Narayanan, P. Strasser
Publisher	Electrochemical Society Inc.
Pages	487-496
Number of pages	10
Edition	17
ISBN (Electronic)	9781607685395
DOIs	https://doi.org/10.1149/06917.0487ecst
State	Published - 2015
Externally published	Yes
Event	Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting - Phoenix, United States Duration: Oct 11 2015 → Oct 15 2015

Publication series

Name	ECS Transactions
Number	17
Volume	69
ISSN (Print)	1938-6737
ISSN (Electronic)	1938-5862

Conference

Conference	Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting
Country/Territory	United States
City	Phoenix
Period	10/11/15 → 10/15/15

Funding

Funders	Funder number
National Science Foundation	CMMI-1265893

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1149/06917.0487ecst

Cite this

Yu, H., Baricci, A., Roller, J., Wang, Y., Casalegno, A., Mustain, W. E., & Maric, R. (2015). Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology. In H. A. Gasteiger, A. Z. Weber, V. K. Ramani, T. F. Fuller, R. A. Mantz, H. Uchida, F. N. Buchi, M. Edmundson, C. Coutanceau, J. M. Fenton, S. Mitsushima, T. J. Schmidt, K. Shinohara, K. Swider-Lyons, D. J. Jones, B. S. Pivovar, K. E. Ayers, K. A. Perry, S. R. Narayanan, & P. Strasser (Eds.), Polymer Electrolyte Fuel Cells 15, PEFC 15 (17 ed., pp. 487-496). (ECS Transactions; Vol. 69, No. 17). Electrochemical Society Inc.. https://doi.org/10.1149/06917.0487ecst

Yu, Haoran ; Baricci, Andrea ; Roller, Justin et al. / Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology. Polymer Electrolyte Fuel Cells 15, PEFC 15. editor / H. A. Gasteiger ; A. Z. Weber ; V. K. Ramani ; T. F. Fuller ; R. A. Mantz ; H. Uchida ; F. N. Buchi ; M. Edmundson ; C. Coutanceau ; J. M. Fenton ; S. Mitsushima ; T. J. Schmidt ; K. Shinohara ; K. Swider-Lyons ; D. J. Jones ; B. S. Pivovar ; K. E. Ayers ; K. A. Perry ; S. R. Narayanan ; P. Strasser. 17. ed. Electrochemical Society Inc., 2015. pp. 487-496 (ECS Transactions; 17).

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title = "Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology",

abstract = "Reactive spray deposition technology (RSDT) is a cost-effective method for producing high performance proton exchange membrane fuel cell (PEMFC) membrane electrode assemblies (MEAs). In this study, we used the RSDT process to deposit catalyst-coated membrane (CCM) with Pt supported on Ketjen Black (KB), multi-wall carbon nanotube (MWCNT) and reducedgraphene oxide (rGO) with ultra-low Pt loading in order to elucidate the influence of the support and Pt dispersion on the catalyst perfromance. The electrochemically active surface area (ECSA), activity for oxygen reduction reaction (ORR) and PEMFC performance are investigated and compared.",

author = "Haoran Yu and Andrea Baricci and Justin Roller and Yang Wang and Andrea Casalegno and Mustain, {William E.} and Radenka Maric",

note = "Publisher Copyright: {\textcopyright} The Electrochemical Society.; Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting ; Conference date: 11-10-2015 Through 15-10-2015",

year = "2015",

doi = "10.1149/06917.0487ecst",

language = "English",

series = "ECS Transactions",

publisher = "Electrochemical Society Inc.",

number = "17",

pages = "487--496",

editor = "Gasteiger, {H. A.} and Weber, {A. Z.} and Ramani, {V. K.} and Fuller, {T. F.} and Mantz, {R. A.} and H. Uchida and Buchi, {F. N.} and M. Edmundson and C. Coutanceau and Fenton, {J. M.} and S. Mitsushima and Schmidt, {T. J.} and K. Shinohara and K. Swider-Lyons and Jones, {D. J.} and Pivovar, {B. S.} and Ayers, {K. E.} and Perry, {K. A.} and Narayanan, {S. R.} and P. Strasser",

booktitle = "Polymer Electrolyte Fuel Cells 15, PEFC 15",

edition = "17",

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Yu, H, Baricci, A, Roller, J, Wang, Y, Casalegno, A, Mustain, WE & Maric, R 2015, Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology. in HA Gasteiger, AZ Weber, VK Ramani, TF Fuller, RA Mantz, H Uchida, FN Buchi, M Edmundson, C Coutanceau, JM Fenton, S Mitsushima, TJ Schmidt, K Shinohara, K Swider-Lyons, DJ Jones, BS Pivovar, KE Ayers, KA Perry, SR Narayanan & P Strasser (eds), Polymer Electrolyte Fuel Cells 15, PEFC 15. 17 edn, ECS Transactions, no. 17, vol. 69, Electrochemical Society Inc., pp. 487-496, Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting, Phoenix, United States, 10/11/15. https://doi.org/10.1149/06917.0487ecst

Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology. / Yu, Haoran; Baricci, Andrea; Roller, Justin et al.
Polymer Electrolyte Fuel Cells 15, PEFC 15. ed. / H. A. Gasteiger; A. Z. Weber; V. K. Ramani; T. F. Fuller; R. A. Mantz; H. Uchida; F. N. Buchi; M. Edmundson; C. Coutanceau; J. M. Fenton; S. Mitsushima; T. J. Schmidt; K. Shinohara; K. Swider-Lyons; D. J. Jones; B. S. Pivovar; K. E. Ayers; K. A. Perry; S. R. Narayanan; P. Strasser. 17. ed. Electrochemical Society Inc., 2015. p. 487-496 (ECS Transactions; Vol. 69, No. 17).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology

AU - Yu, Haoran

AU - Baricci, Andrea

AU - Roller, Justin

AU - Wang, Yang

AU - Casalegno, Andrea

AU - Mustain, William E.

AU - Maric, Radenka

N1 - Publisher Copyright: © The Electrochemical Society.

PY - 2015

Y1 - 2015

N2 - Reactive spray deposition technology (RSDT) is a cost-effective method for producing high performance proton exchange membrane fuel cell (PEMFC) membrane electrode assemblies (MEAs). In this study, we used the RSDT process to deposit catalyst-coated membrane (CCM) with Pt supported on Ketjen Black (KB), multi-wall carbon nanotube (MWCNT) and reducedgraphene oxide (rGO) with ultra-low Pt loading in order to elucidate the influence of the support and Pt dispersion on the catalyst perfromance. The electrochemically active surface area (ECSA), activity for oxygen reduction reaction (ORR) and PEMFC performance are investigated and compared.

AB - Reactive spray deposition technology (RSDT) is a cost-effective method for producing high performance proton exchange membrane fuel cell (PEMFC) membrane electrode assemblies (MEAs). In this study, we used the RSDT process to deposit catalyst-coated membrane (CCM) with Pt supported on Ketjen Black (KB), multi-wall carbon nanotube (MWCNT) and reducedgraphene oxide (rGO) with ultra-low Pt loading in order to elucidate the influence of the support and Pt dispersion on the catalyst perfromance. The electrochemically active surface area (ECSA), activity for oxygen reduction reaction (ORR) and PEMFC performance are investigated and compared.

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DO - 10.1149/06917.0487ecst

M3 - Conference contribution

AN - SCOPUS:84946065742

T3 - ECS Transactions

SP - 487

EP - 496

BT - Polymer Electrolyte Fuel Cells 15, PEFC 15

A2 - Gasteiger, H. A.

A2 - Weber, A. Z.

A2 - Ramani, V. K.

A2 - Fuller, T. F.

A2 - Mantz, R. A.

A2 - Uchida, H.

A2 - Buchi, F. N.

A2 - Edmundson, M.

A2 - Coutanceau, C.

A2 - Fenton, J. M.

A2 - Mitsushima, S.

A2 - Schmidt, T. J.

A2 - Shinohara, K.

A2 - Swider-Lyons, K.

A2 - Jones, D. J.

A2 - Pivovar, B. S.

A2 - Ayers, K. E.

A2 - Perry, K. A.

A2 - Narayanan, S. R.

A2 - Strasser, P.

PB - Electrochemical Society Inc.

T2 - Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting

Y2 - 11 October 2015 through 15 October 2015

ER -

Yu H, Baricci A, Roller J, Wang Y, Casalegno A, Mustain WE et al. Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology. In Gasteiger HA, Weber AZ, Ramani VK, Fuller TF, Mantz RA, Uchida H, Buchi FN, Edmundson M, Coutanceau C, Fenton JM, Mitsushima S, Schmidt TJ, Shinohara K, Swider-Lyons K, Jones DJ, Pivovar BS, Ayers KE, Perry KA, Narayanan SR, Strasser P, editors, Polymer Electrolyte Fuel Cells 15, PEFC 15. 17 ed. Electrochemical Society Inc. 2015. p. 487-496. (ECS Transactions; 17). doi: 10.1149/06917.0487ecst

Ultra-low Pt loading catalyst layers for PEMFC using reactive spray deposition technology

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UN SDGs

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