Two-in-one: Construction of hydroxyl and imidazolium-bifunctionalized ionic networks in one-pot toward synergistic catalytic CO2 fixation

Yadong Zhang, Guojian Chen, Lei Wu, Ke Liu, Hu Zhong, Zhouyang Long, Minman Tong, Zhenzhen Yang, Sheng Dai

Research output: Contribution to journalArticlepeer-review

113 Scopus citations

Abstract

A succinct strategy was demonstrated for constructing a hydroxyl group and imidazolium-bifunctionalized ionic network via a one-pot quaternization. Key to success lies in the rational design of multi-imidazole precursor and hydroxyl-containing counterpart. Unique properties of the resultant ionic network render its high catalytic efficiency toward CO2 fixation under ambient conditions.

Original languageEnglish
Pages (from-to)3309-3312
Number of pages4
JournalChemical Communications
Volume56
Issue number22
DOIs
StatePublished - Mar 18 2020

Funding

This work was supported by the National Natural Science Foundation of China (21603089, 21706106 and 21503098), Natural Science Foundation of Jiangsu Province (BK20160209), and Natural Science Foundation of Jiangsu Higher Education Institutions of China (16KJB150014). ZY and SD were supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy.

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