Time-resolved measurements of emission transients by mass spectrometry

William P. Partridge, John M.E. Storey, Samuel A. Lewis, Robert W. Smithwick, Gerald L. Devault, Michael J. Cunningham, Neal W. Currier, Thomas M. Yonushonis

Research output: Contribution to journalConference articlepeer-review

41 Scopus citations

Abstract

High-speed diagnostics capable of accurately resolving emission transients are required to provide the most detailed understanding and optimization of active exhaust-emissions-treatment processes, such as NOX adsorbers. A portable, mass-spectrometry-based instrument with high temporal resolution, linear response and broad dynamic range is described. This instrument provides transient-concentration measurement capability for many relevant exhaust species including total NOX. In applications for evaluation of NO X-adsorber systems using heavy-duty diesel engines, the instrument revealed relevant emission transients not previously resolved with conventional analyzers. Specifically, the instrument resolved transient emissions associated with the competition between desorption and reduction rates. The temporal resolution of the instruments is sufficient to resolve kinetic rates of the NOX-adsorber system.

Original languageEnglish
JournalSAE Technical Papers
DOIs
StatePublished - 2000
EventInternational Fall Fuels and Lubricants Meeting and Exposition - Baltimore, MD, United States
Duration: Oct 16 2000Oct 19 2000

Fingerprint

Dive into the research topics of 'Time-resolved measurements of emission transients by mass spectrometry'. Together they form a unique fingerprint.

Cite this