TY - JOUR
T1 - Time-resolved magneto-optical effects in the altermagnet candidate MnTe
AU - Gray, Isaiah
AU - Deng, Qinwen
AU - Tian, Qi
AU - Chilcote, Michael
AU - Dodge, J. Steven
AU - Brahlek, Matthew
AU - Wu, Liang
N1 - Publisher Copyright:
© 2024 Author(s).
PY - 2024/11/18
Y1 - 2024/11/18
N2 - α -MnTe is an antiferromagnetic semiconductor with above room temperature T N = 310 K, which is promising for spintronic applications. Recently, it was reported to be an altermagnet, containing bands with momentum-dependent spin splitting; time-resolved experimental probes of MnTe are, therefore, important both for understanding novel magnetic properties and potential device applications. We investigate ultrafast spin dynamics in epitaxial MnTe(001)/InP(111) thin films using pump-probe magneto-optical measurements in the Kerr configuration. At room temperature, we observe an oscillation mode at 55 GHz that does not appear at zero magnetic field. Combining field and polarization dependence, we identify this mode as a magnon, likely originating from inverse stimulated Raman scattering. Magnetic field-dependent oscillations persist up to at least 335 K, which could reflect coupling to known short-range magnetic order in MnTe above T N . Additionally, we observe two optical phonons at 3.6 and 4.2 THz, which broaden and redshift with increasing temperature.
AB - α -MnTe is an antiferromagnetic semiconductor with above room temperature T N = 310 K, which is promising for spintronic applications. Recently, it was reported to be an altermagnet, containing bands with momentum-dependent spin splitting; time-resolved experimental probes of MnTe are, therefore, important both for understanding novel magnetic properties and potential device applications. We investigate ultrafast spin dynamics in epitaxial MnTe(001)/InP(111) thin films using pump-probe magneto-optical measurements in the Kerr configuration. At room temperature, we observe an oscillation mode at 55 GHz that does not appear at zero magnetic field. Combining field and polarization dependence, we identify this mode as a magnon, likely originating from inverse stimulated Raman scattering. Magnetic field-dependent oscillations persist up to at least 335 K, which could reflect coupling to known short-range magnetic order in MnTe above T N . Additionally, we observe two optical phonons at 3.6 and 4.2 THz, which broaden and redshift with increasing temperature.
UR - http://www.scopus.com/inward/record.url?scp=85209880887&partnerID=8YFLogxK
U2 - 10.1063/5.0244878
DO - 10.1063/5.0244878
M3 - Article
AN - SCOPUS:85209880887
SN - 0003-6951
VL - 125
JO - Applied Physics Letters
JF - Applied Physics Letters
IS - 21
M1 - 212404
ER -