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Sustainable biobased composites: From raw materials to recycling

  • Ya Tang
  • , Zhijing Zhan
  • , Shuvodeep De
  • , Umesh Marathe
  • , Halil Tekinalp
  • , Soydan Ozcan
  • , Wen Dong
  • , Qing Jin
  • , Xianhui Zhao
  • , Yan Li

Research output: Contribution to journalReview articlepeer-review

4 Scopus citations

Abstract

Biobased composites, which consist of natural fibers and biobased polymer binders, are gaining traction due to their renewability, low carbon footprint, lightweight nature, multifunctionality, and potential recycling capabilities. Despite their promise, these materials face challenges such as moisture sensitivity, thermal degradation, and limited durability, often due to weak fiber-matrix interfaces. Addressing these challenges and advancing their development requires a comprehensive understanding of material constituents, interfacial behavior, processing techniques, and lifecycle performance. However, existing reviews remain scattered, typically focusing on a single aspect, such as material development and fabrication methods. In this paper, we provide an integrated overview of the biobased composites across the full lifecycle, from raw material selection and interface treatments to scalable manufacturing, recycling, and end-use applications. We summarize various surface treatment methods used to enhance the mechanical properties, durability, and functionality of biocomposites, and systematically compare their performance, cost, and biodegradability. Scalable production techniques that affect the structure and properties of biocomposite products are compared. End-of-life management routes, including mechanical, chemical, and thermal recycling, are evaluated with respect to cost and efficiency. The industrial applications and future research directions are also explored to promote the wider adoption of biobased composites across key sectors such as automotive, aerospace, and construction.

Original languageEnglish
Article number113188
JournalComposites Part B: Engineering
Volume311
DOIs
StatePublished - Feb 15 2026

Funding

The authors acknowledge the support from the Arthur L. Irving Institute for Energy and Society, Thayer School of Engineering at Dartmouth College. The authors also acknowledge the support from the US Department of Energy (DOE), Bioenergy Technologies Office. This manuscript was authored in part by UT-Battelle LLC under contract DE-AC05-00OR22725 with DOE. The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). This research was supported in part by an appointment to the Oak Ridge National Laboratory GRO Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education.

Keywords

  • Biopolymer
  • Circular bioeconomy
  • Composite
  • Natural fiber
  • Surface treatment

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