Structure and magnetic properties of the pyrochlore iridate Y 2Ir 2O 7

M. C. Shapiro, Scott C. Riggs, M. B. Stone, C. R. De La Cruz, S. Chi, A. A. Podlesnyak, I. R. Fisher

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Abstract

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y 2Ir 2O 7. Temperature-dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign of any structural or disorder-induced phase transition was observed over the entire temperature range. In addition, no sign of magnetic long-range order was observed to within the sensitivity of the instrumentation. These measurements do not rule out long-range magnetic order, but the neutron-powder-diffraction structural refinements do put an upper bound for the ordered iridium moment of ∼0.2 μ B/Ir (for a magnetic structure with wave vector Q*0) or ∼0.5 μ B/Ir (for Q=0).

Original languageEnglish
Article number214434
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume85
Issue number21
DOIs
StatePublished - Jun 26 2012

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