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Step-loaded creep testing of Zircaloy-4 cladding at higher temperatures in the α-phase

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Abstract

A refined understanding of zirconium-based cladding thermomechanical performance during rapid transients is essential for enhancing the safety and operation of light-water reactors. Traditional models for zirconium alloys under accident conditions generally assume that creep dominates fuel cladding performance. These historic models have largely remained unchanged and serve as the basis for safety criteria development. As the U.S. nuclear industry pursues higher burnup levels, the increased release of fission gases during transients raises the risk of cladding failure in the low-temperature hcp α-phase, making the fidelity of these models of greater importance. Creep testing was conducted from 550–700°C with 25–120 MPa applied hoop stresses to investigate Zircaloy-4 deformation at accident-relevant temperatures in the α-phase. Step-loading was employed to capture creep behavior across a wide stress range from a single sample. The stress-strain rate data at higher temperatures (650 and 700°C) were well-described by isotropic versions of the Erbacher and Kaddour models, while the lower temperature data (550 and 600°C) were underpredicted by both anisotropic and isotropic model variants. Greater strain rates during the initial loading step at 650 and 700°C were attributed to recrystallization and grain growth of sub-micron crystallites. Yet, texture analysis revealed the basal split texture remained after testing. These observations produced results suggesting Zircaloy-4 claddings experience higher creep rates across the α-phase than previously thought, possibly related to dynamic anisotropy due to temperature dependent activation of deformation mechanisms, effects of biaxial loading, and variation in material condition between the current testing used in previous model development.

Original languageEnglish
Article number120821
JournalActa Materialia
Volume288
DOIs
StatePublished - Apr 15 2025

Funding

The authors would like to thank B. Garrison and P. Doyle for advice and guidance regarding the data and manuscript, A. Godfrey for characterization, and B. Johnston and J. Wade for help conducting the tests needed for the study. Electron microscopy was performed using ORNL's Low Activation Materials Development and Analysis (LAMDA) laboratory. This work was performed as a part of the Advanced Fuels Campaign directed by the United States Department of Energy Office of Nuclear Energy.

Keywords

  • Accident
  • Creep
  • Isotropy
  • Zirconium fuel cladding

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