Abstract
Altermagnetism is a newly discovered magnetic phase, characterized by nonrelativistic spin splitting that has been experimentally observed. Here, we introduce a framework dubbed "spin-orbital altermagnetism"to achieve spin-orbital textures in altermagnetic materials. We identify two distinct classes of spin-orbital altermagnetism: intrinsic and extrinsic. The intrinsic type emerges from symmetry-compensated magnetic orders with spontaneously broken parity-time symmetry, while the extrinsic type stems from translational symmetry breaking between sublattices, as exemplified by the Jahn-Teller-driven structural phase transition. In addition to directly measuring the spin-orbital texture, we propose spin conductivity and spin-resolved orbital polarization as effective methods for detecting these altermagnets. Additionally, a symmetry-breaking mechanism induces weak spin magnetization, further revealing the peculiar feature of spin-orbital altermagnetism. We also utilize the staggered susceptibility to illustrate a potential realization of this phase in a two-orbital interacting system. Our Letter provides a new platform to explore spin-orbital locked physics, extending the materials classes that may display complex spin textures from the standard 4d-5d compounds to 3d compounds.
| Original language | English |
|---|---|
| Article number | 176705 |
| Journal | Physical Review Letters |
| Volume | 135 |
| Issue number | 17 |
| DOIs | |
| State | Published - Oct 24 2025 |
Funding
We thank K.-J. Yang, H.-M. Yi, M. Zeng, and C.-X. Liu for helpful discussions. We thank C. Lu for discussions and collaborations on closely related projects. L. H. H. is supported by National Key R&D Program of China (Grant No. 2022YFA1402200), the National Natural Science Foundation of China (Grant No. 12034017). Z. M. W. and D. H. X. were supported in part by the NSFC (Grants No. 12074108, No. 12474151, and No. 12347101), the Natural Science Foundation of Chongqing (Grant No. CSTB2022NSCQ-MSX0568). S. B. Z. acknowledges the support of the start-up fund at Hefei National Laboratory, the Innovation Program for Quantum Science and Technology (Grant No. 2021ZD0302800), and the National Natural Science Foundation of China (Grant No. 12488101). Z. M. W. and L. H. H. is supported by the start-up of Zhejiang University and the Fundamental Research Funds for the Central Universities (Grant No. 226-2024-00068).