Spin-flop phase in a honeycomb antiferromagnet Mn0.84Mg0.16TiO3

Shin Ichi Shamoto, Hiroki Yamauchi, Kazuhiko Ikeuchi, Min Kai Lee, Lieh Jeng Chang, V. Ovidiu Garlea, In Yong Hwang, Kee Hwan Lee, Jae Ho Chung

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Abstract

The spin-flop phase of a honeycomb antiferromagnet of Mn0.84Mg0.16TiO3 has been studied under magnetic field along normal direction to the honeycomb plane by neutron scattering. With increasing a magnetic field from 0 to 5 T, the inelastic scattering intensity increased by 1.5 times at (1 0 0), where the magnetic structure was found to be collinear-antiferromagnet with the spin parallel to [1 1 0] direction. The spin direction is consistent with a 1.5 times increase of the inelastic intensity. The negligible energy difference between K and KA points suggests small values for both Dzyaloshinskii-Moriya interaction and bond-dependent symmetric anisotropic exchange interaction in this material.

Original languageEnglish
Article number093703
JournalJournal of the Physical Society of Japan
Volume90
Issue number9
DOIs
StatePublished - Sep 15 2021

Funding

Acknowledgments S.S. thanks for the invaluable discussion with Professors S. Hayami and M. Akatsu. K.I. thanks for the travel expense support from ISSP, Univ. Tokyo. This research was partly supported by the National Research Foundation of Korea (Grant No. 2020K1A3A7A09077712). This research used resources at the Spallation Neutron Source, DOE Office of Science User Facilities operated by the Oak Ridge National Laboratory. S.S. thanks for the invaluable discussion with Professors S. Hayami and M. Akatsu. K.I. thanks for the travel expense support from ISSP, Univ. Tokyo. This research was partly supported by the National Research Foundation of Korea (Grant No. 2020K1A3A7A09077712). This research used resources at the Spallation Neutron Source, DOE Office of Science User Facilities operated by the Oak Ridge National Laboratory.

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