Abstract
Kagome-lattice materials have attracted tremendous interest due to the broad prospect for seeking superconductivity, quantum spin liquid states, and topological electronic structures. Among them, the transition-metal kagome lattices are high-profile objects for the combination of topological properties, rich magnetism, and multiple-orbital physics. Here we report an inelastic neutron scattering study on the spin dynamics of a kagome-lattice antiferromagnetic metal Fe0.89Co0.11Sn. Although the magnetic excitations can be observed up to ∼250 meV, well-defined spin waves are only identified below ∼90 meV and can be modeled using Heisenberg exchange with ferromagnetic in-plane nearest-neighbor coupling J1, in-plane next-nearest-neighbor coupling J2, and antiferromagnetic (AFM) interlayer coupling Jc under linear spin-wave theory. Above ∼90 meV, the spin waves enter the itinerant Stoner continuum and become highly damped particle-hole excitations. At the K point of the Brillouin zone, we reveal a possible band crossing of the spin wave, which indicates a potential Dirac magnon. Our results uncover the evolution of the spin excitations from the planar AFM state to the axial AFM state in Fe0.89Co0.11Sn, solve the magnetic Hamiltonian for both states, and confirm the significant influence of the itinerant magnetism on the spin excitations.
Original language | English |
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Article number | 214436 |
Journal | Physical Review B |
Volume | 106 |
Issue number | 21 |
DOIs | |
State | Published - Dec 1 2022 |
Funding
We thank Dr. Victor Fanelli for help with the experiment at the SEQUOIA spectrometer, Dr. Jong Keum for help with the x-ray Laue measurements, and Dr. Matthew Stone for suggestions about the neutron beam time application. Work at Oak Ridge National Laboratory (ORNL) was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. H.L. was supported by the National Key R&D Program of China (Grants No. 2018YFE0202600 and No. 2022YFA1403800), the Beijing Natural Science Foundation (Grant No. Z200005), and the National Natural Science Foundation of China (12274459). This research used resources at the Spallation Neutron Source, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory. X-ray Laue measurements were conducted at the Center for Nanophase Materials Sciences (CNMS) (CNMS2019-R18) at ORNL, which is a DOE Office of Science User Facility.
Funders | Funder number |
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U.S. Department of Energy | |
Office of Science | |
Basic Energy Sciences | |
Oak Ridge National Laboratory | |
Division of Materials Sciences and Engineering | |
National Natural Science Foundation of China | 12274459 |
Natural Science Foundation of Beijing Municipality | Z200005 |
National Key Research and Development Program of China | 2022YFA1403800, 2018YFE0202600 |