Solvent-Free Synthesis of CuO/HKUST-1 Composite and Its Photocatalytic Application

Ming Jin; Xuefeng Qian; Junkuo Gao; Jihua Chen; Dale K. Hensley; Hoi Chun Ho; Rebecca J. Percoco; Christopher M. Ritzi; Yanfeng Yue

doi:10.1021/acs.inorgchem.9b00362

Solvent-Free Synthesis of CuO/HKUST-1 Composite and Its Photocatalytic Application

Ming Jin, Xuefeng Qian, Junkuo Gao, Jihua Chen, Dale K. Hensley, Hoi Chun Ho, Rebecca J. Percoco, Christopher M. Ritzi, Yanfeng Yue

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57 Scopus citations

Abstract

A metal-organic framework (MOF) is one kind of crystalline microporous material and is increasingly used as a host of catalytically active guests. Nanostructured materials supported on MOFs have presented enhanced catalytic activity and stability. Templates or several steps are essential to the synthesis of MOF composites. Simple and effective MOF synthesis methods are still challenging. Nanosized copper oxide particles in MOF composites, described as nanosized CuO@HKUST-1, were prepared by a facile solvent-free reaction. These series of CuO@HKUST-1 composites exhibited excellent photocatalytic activity for production of hydrogen and methylene blue (MB) degradation under visible light. This synthesis method provides an effective way to fabricate MOF-related nanocomposite catalysts.

Original language	English
Pages (from-to)	8332-8338
Number of pages	7
Journal	Inorganic Chemistry
Volume	58
Issue number	13
DOIs	https://doi.org/10.1021/acs.inorgchem.9b00362
State	Published - Jul 1 2019

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title = "Solvent-Free Synthesis of CuO/HKUST-1 Composite and Its Photocatalytic Application",

abstract = "A metal-organic framework (MOF) is one kind of crystalline microporous material and is increasingly used as a host of catalytically active guests. Nanostructured materials supported on MOFs have presented enhanced catalytic activity and stability. Templates or several steps are essential to the synthesis of MOF composites. Simple and effective MOF synthesis methods are still challenging. Nanosized copper oxide particles in MOF composites, described as nanosized CuO@HKUST-1, were prepared by a facile solvent-free reaction. These series of CuO@HKUST-1 composites exhibited excellent photocatalytic activity for production of hydrogen and methylene blue (MB) degradation under visible light. This synthesis method provides an effective way to fabricate MOF-related nanocomposite catalysts.",

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AU - Jin, Ming

AU - Qian, Xuefeng

AU - Gao, Junkuo

AU - Chen, Jihua

AU - Hensley, Dale K.

AU - Ho, Hoi Chun

AU - Percoco, Rebecca J.

AU - Ritzi, Christopher M.

AU - Yue, Yanfeng

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AB - A metal-organic framework (MOF) is one kind of crystalline microporous material and is increasingly used as a host of catalytically active guests. Nanostructured materials supported on MOFs have presented enhanced catalytic activity and stability. Templates or several steps are essential to the synthesis of MOF composites. Simple and effective MOF synthesis methods are still challenging. Nanosized copper oxide particles in MOF composites, described as nanosized CuO@HKUST-1, were prepared by a facile solvent-free reaction. These series of CuO@HKUST-1 composites exhibited excellent photocatalytic activity for production of hydrogen and methylene blue (MB) degradation under visible light. This synthesis method provides an effective way to fabricate MOF-related nanocomposite catalysts.

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Solvent-Free Synthesis of CuO/HKUST-1 Composite and Its Photocatalytic Application

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