Abstract
Topological quantum phases are largely understood in weakly correlated systems, which have identified various quantum phenomena, such as the spin Hall effect, protected transport of helical fermions, and topological superconductivity. Robust ferromagnetic order in correlated topological materials particularly attracts attention, as it can provide a versatile platform for novel quantum devices. Here, a singular Hall response arising from a unique band structure of flat topological nodal lines in combination with electron correlation in a van der Waals ferromagnetic semimetal, Fe3GaTe2, with a high Curie temperature of Tc = 347 K is reported. High anomalous Hall conductivity violating the conventional scaling, resistivity upturn at low temperature, and a large Sommerfeld coefficient are observed in Fe3GaTe2, which implies heavy fermion features in this ferromagnetic topological material. The scanning tunneling microscopy, circular dichroism in angle-resolved photoemission spectroscopy, and theoretical calculations support the original electronic features of the material. Thus, low-dimensional Fe3GaTe2 with electronic correlation, topology, and room-temperature ferromagnetic order appears to be a promising candidate for robust quantum devices.
Original language | English |
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Article number | 2402040 |
Journal | Advanced Materials |
Volume | 36 |
Issue number | 31 |
DOIs | |
State | Published - Aug 1 2024 |
Funding
This work was supported by the Samsung Research Funding & Incubation Center of Samsung Electronics under Project No. SRFC\u2010MA1701\u201052 and the NRF (No. RS\u20102024\u201000340377). J.O. and Y.Y. acknowledge the National Research Foundation of Korea (NRF) Grants funded by the Korean Government (MSIT) (Grant No. RS\u20102023\u201000208179). J.P. and C.K. were supported by NRF (No. 2022R1A3B1077234). J.C. and Y.K. were supported by the National Research Foundation (NRF) of Korea funded by the Korean government (grant. nos. 2021R1A2C1013119, 2020K1A3A7A09080366) and National Measurement Standard Services and Technical Services for SME funded by the Korea Research Institute of Standards and Science (grant No. KRISS \u2010 2023 \u2010 GP2023\u20100015). Y.\u2010G.K., D.H.D.L., D.H.K., and M.J.H. were supported by the National Research Foundation of Korea (NRF) grant funcded by the Korea government (MSIT) (Grant No. RS\u20102023\u201000253716). The electron microscopy experiments were conducted using a double Cs corrected Titan cubed G2 60\u2010300 (FEI) equipment at the KAIST Analysis Center for Research Advancement (KARA). Excellent support by Tae Woo Lee, Jin\u2010Seok Choi, and the staff of KARA is gratefully acknowledged. The electron microscopy data analyses were partially supported by the KAIST Quantum Research Core Facility Center (KBSI\u2013NFEC grant funded by the Korea government MSIT, Grant No. PG2022004\u201009). The ARPES experiments were conducted at the beamline 4.0.3 (MERLIN) of the Advanced Light Source (ALS). The use of ALS is supported by the Office of Basic Energy Sciences of the US DOE under contract No. DE\u2010AC02\u201005CH11231.
Keywords
- angle-resolved photoemission spectroscopy
- anomalous Hall conductivity
- correlated states
- ferromagnetism
- topological materials