Single-atom dynamics in scanning transmission electron microscopy

Rohan Mishra, Ryo Ishikawa, Andrew R. Lupini, Stephen J. Pennycook

Research output: Contribution to journalReview articlepeer-review

32 Scopus citations

Abstract

The correction of aberrations in the scanning transmission electron microscope (STEM) has simultaneously improved both spatial and temporal resolution, making it possible to capture the dynamics of single atoms inside materials, and resulting in new insights into the dynamic behavior of materials. In this article, we describe the different beam-matter interactions that lead to atomic excitations by transferring energy and momentum. We review recent examples of sequential STEM imaging to demonstrate the dynamic behavior of single atoms both within materials, at dislocations, at grain and interface boundaries, and on surfaces. We also discuss the effects of such dynamic behavior on material properties. We end with a summary of ongoing instrumental and algorithm developments that we anticipate will improve the temporal resolution significantly, allowing unprecedented insights into the dynamic behavior of materials at the atomic scale.

Original languageEnglish
Pages (from-to)644-652
Number of pages9
JournalMRS Bulletin
Volume42
Issue number9
DOIs
StatePublished - Sep 1 2017

Funding

R.M. acknowledges financial support through the National Science Foundation (Grant No. DMREF-1729787). Research at Oak Ridge National Laboratory was supported by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences.

FundersFunder number
Office of Basic Energy Sciences
National Science FoundationDMREF-1729787, 1729787
Division of Materials Sciences and Engineering
Japan Society for the Promotion of Science17K18974, 17H06094

    Keywords

    • diffusion
    • dislocations
    • grain boundaries
    • phase transformation

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