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Self-assembly of wood-based shape memory composites triggered by solar-thermal energy

  • Mengtian Gan
  • , Xiao Zhang
  • , Amber M. Hubbard
  • , Caitlyn M. Clarkson
  • , Thomas Wei
  • , Dinesh K. Patel
  • , Lining Yao

Research output: Contribution to journalArticlepeer-review

Abstract

Transporting and assembling large, complex structures poses significant challenges due to their size, geometry, and cost. Additionally, the installation sites are often inaccessible or hazardous for humans, necessitating self-assembling capabilities in these structures. To mitigate these challenges, we propose using 3D printing materials with shape memory effect (SME) for both transport and construction. This approach involves developing 3D modular components into flat sheets for easier transportation, and then self-assembling into 3D structures on-site using solar energy. To gain a deeper understanding of the factors influencing material memory performance, we have chosen a composite PLA/WF, which is polylactic acid (PLA) with 20 wt% wood flour (WF) for this purpose, leveraging its high tensile modulus at 0.966 GPa, low cost, and sustainability. Printed shapes with this material can maintain a recovery ratio over 90% after 3 cycles. While traditional composites fillers (e.g. glass or carbon fiber) are added to enhance mechanical and thermal properties, the addition of bio-based fillers like WF accomplish similar goals without compromising sustainability. We conducted multiple experiments to demonstrate how environmental conditions (i.e. temperature) maximize the material’s SME. Although still at an early stage, this study provides initial insights into bridging the gap between the small-scale nature of shape memory polymers (SMPs) and their potential for large-scale additive manufacturing, addressing a critical need for efficient and sustainable construction. In the long term, we hope our study contributes to the design vision of utilizing SMPs for transportation, assembly, and deployment of complex structures, providing a new pathway for sustainable construction and transportation of large-scale structures to hard-to-access locations such as disaster-affected areas and remote deserts, etc.

Original languageEnglish
Article number125025
JournalSmart Materials and Structures
Volume34
Issue number12
DOIs
StatePublished - Dec 1 2025

Funding

This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). This research was supported by the U.S. Department of Energy (DOE), Advanced Materials and Manufacturing Technologies Office and used resources at the Manufacturing Demonstration Facility at Oak Ridge National Laboratory, a User Facility of DOE’s Office of Energy Efficiency and Renewable Energy. The authors acknowledge the support from the US Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, Advanced Materials and Manufacturing Office under CPS 848 Agreement 35714, and Oak Ridge National Laboratory/University of Maine Hub & Spoke Program team. The authors also acknowledge support from the National Science Foundation Career Grant IIS-2427455, 2427457 and 2427553 (LY). Microscopy studies were completed at the Center for Nanophase Materials Sciences, a DOE Office of Science User Facility. The authors would also like to thank Dr Katie Copenhaver for SEM imaging assistance.

Keywords

  • 4D printing
  • PLA
  • assembly
  • deployment
  • morphing
  • shape memory effect
  • wood flour

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