Scanning nano-Raman spectroscopy of semiconducting structures

R. D. Hartschuh, N. Lee, D. Mehtani, A. Kisliuk, M. D. Foster, A. P. Sokolov, J. F. Maguire

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

4 Scopus citations

Abstract

Tip-enhanced Raman spectroscopy (TERS) using side illumination is a promising spectroscopic tool for nanoscale characterization of chemical composition, structure, stresses and conformational states of non-transparent samples. Recent progress has shown signal enhancements for a variety of samples, including break-through enhancements of semiconductors. In this work, optimization of the polarization geometry increases contrast between near-field and far-field signals on Si and improves imaging quality. Two-dimensional images of semiconductor nanostructures show reasonable agreement between topographical and TERS images. These recent TERS results using both silver- and gold-coated tips demonstrate localization of the Raman enhancement to within approximately 20 nm of the tip. Also, the enhanced Raman signal of a strained Si layer is separated from an underlying Si substrate, which is encouraging for potential strain distribution analysis of silicon nanostructures.

Original languageEnglish
Title of host publicationPlasmonics
Subtitle of host publicationNanoimaging, Nanofabrication, and their Applications II
DOIs
StatePublished - 2006
Externally publishedYes
EventPlasmonics: Nanoimaging, Nanofabrication, and their Applications II - San Diego, CA, United States
Duration: Aug 16 2006Aug 17 2006

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
Volume6324
ISSN (Print)0277-786X

Conference

ConferencePlasmonics: Nanoimaging, Nanofabrication, and their Applications II
Country/TerritoryUnited States
CitySan Diego, CA
Period08/16/0608/17/06

Keywords

  • Apertureless near-field
  • Contrast
  • Imaging
  • Polarization
  • Scanning nano-Raman spectroscopy (SNRS)
  • Side-illumination
  • Strained silicon
  • Sub-wavelength resolution
  • Surface plasmon resonance
  • Tip-enhanced Raman spectroscopy (TERS)

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