S=2 quasi-one-dimensional spin waves in CrCl2

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Abstract

We examine the magnetic excitation spectrum in the S=2 Heisenberg antiferromagnet CrCl2. Inelastic neutron scattering measurements on powder samples are able to determine the significant exchange interactions in this system. A large anisotropy gap is observed in the spectrum below the Néel temperature and the ratio of the two largest exchange constants is Jc/Jb=9.1±2.2. However, no sign of a gapped quantum spin liquid excitation was found in the paramagnetic phase.

Original languageEnglish
Article number104413
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume88
Issue number10
DOIs
StatePublished - Sep 16 2013

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