Robust A-Type Order and Spin-Flop Transition on the Surface of the Antiferromagnetic Topological Insulator MnBi2Te4

Paul M. Sass, Jinwoong Kim, David Vanderbilt, Jiaqiang Yan, Weida Wu

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80 Scopus citations

Abstract

Here, we present microscopic evidence of the persistence of uniaxial A-type antiferromagnetic order to the surface layers of MnBi2Te4 single crystals using magnetic force microscopy. Our results reveal termination-dependent magnetic contrast across both surface step edges and domain walls, which can be screened by thin layers of soft magnetism. The robust surface A-type order is further corroborated by the observation of termination-dependent surface spin-flop transitions, which have been theoretically proposed decades ago. Our results not only provide key ingredients for understanding the electronic properties of the antiferromagnetic topological insulator MnBi2Te4, but also open a new paradigm for exploring intrinsic surface metamagnetic transitions in natural antiferromagnets.

Original languageEnglish
Article number037201
JournalPhysical Review Letters
Volume125
Issue number3
DOIs
StatePublished - Jul 17 2020

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