Reversible Control of Interfacial Magnetism through Ionic-Liquid-Assisted Polarization Switching

Andreas Herklotz; Er Jia Guo; Anthony T. Wong; Tricia L. Meyer; Sheng Dai; T. Zac Ward; Ho Nyung Lee; Michael R. Fitzsimmons

doi:10.1021/acs.nanolett.6b04949

Reversible Control of Interfacial Magnetism through Ionic-Liquid-Assisted Polarization Switching

Andreas Herklotz
, Er Jia Guo
, Anthony T. Wong
, Tricia L. Meyer
, Sheng Dai
, T. Zac Ward
, Ho Nyung Lee
, Michael R. Fitzsimmons

Research output: Contribution to journal › Article › peer-review

32 Scopus citations

Abstract

The ability to control magnetism of materials via electric field enables a myriad of technological innovations in information storage, sensing, and computing. We use ionic-liquid-assisted ferroelectric switching to demonstrate reversible modulation of interfacial magnetism in a multiferroic heterostructure composed of ferromagnetic (FM) La_0.8Sr_0.2MnO₃ and ferroelectric (FE) PbZr_0.2Ti_0.8O₃. It is shown that ionic liquids can be used to persistently and reversibly switch a large area of a FE film. This is a prerequisite for polarized neutron reflectometry (PNR) studies that are conducted to directly probe magnetoelectric coupling of the FE polarization to the interfacial magnetization.

Original language	English
Pages (from-to)	1665-1669
Number of pages	5
Journal	Nano Letters
Volume	17
Issue number	3
DOIs	https://doi.org/10.1021/acs.nanolett.6b04949
State	Published - Mar 8 2017

Keywords

Magnetoelectric coupling
ferroelectric field effect
ionic liquid gating
polarized neutron reflectometry
strongly correlated oxide

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10.1021/acs.nanolett.6b04949

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title = "Reversible Control of Interfacial Magnetism through Ionic-Liquid-Assisted Polarization Switching",

abstract = "The ability to control magnetism of materials via electric field enables a myriad of technological innovations in information storage, sensing, and computing. We use ionic-liquid-assisted ferroelectric switching to demonstrate reversible modulation of interfacial magnetism in a multiferroic heterostructure composed of ferromagnetic (FM) La0.8Sr0.2MnO3 and ferroelectric (FE) PbZr0.2Ti0.8O3. It is shown that ionic liquids can be used to persistently and reversibly switch a large area of a FE film. This is a prerequisite for polarized neutron reflectometry (PNR) studies that are conducted to directly probe magnetoelectric coupling of the FE polarization to the interfacial magnetization.",

keywords = "Magnetoelectric coupling, ferroelectric field effect, ionic liquid gating, polarized neutron reflectometry, strongly correlated oxide",

author = "Andreas Herklotz and Guo, \{Er Jia\} and Wong, \{Anthony T.\} and Meyer, \{Tricia L.\} and Sheng Dai and Ward, \{T. Zac\} and Lee, \{Ho Nyung\} and Fitzsimmons, \{Michael R.\}",

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T1 - Reversible Control of Interfacial Magnetism through Ionic-Liquid-Assisted Polarization Switching

AU - Herklotz, Andreas

AU - Guo, Er Jia

AU - Wong, Anthony T.

AU - Meyer, Tricia L.

AU - Dai, Sheng

AU - Ward, T. Zac

AU - Lee, Ho Nyung

AU - Fitzsimmons, Michael R.

PY - 2017/3/8

Y1 - 2017/3/8

N2 - The ability to control magnetism of materials via electric field enables a myriad of technological innovations in information storage, sensing, and computing. We use ionic-liquid-assisted ferroelectric switching to demonstrate reversible modulation of interfacial magnetism in a multiferroic heterostructure composed of ferromagnetic (FM) La0.8Sr0.2MnO3 and ferroelectric (FE) PbZr0.2Ti0.8O3. It is shown that ionic liquids can be used to persistently and reversibly switch a large area of a FE film. This is a prerequisite for polarized neutron reflectometry (PNR) studies that are conducted to directly probe magnetoelectric coupling of the FE polarization to the interfacial magnetization.

AB - The ability to control magnetism of materials via electric field enables a myriad of technological innovations in information storage, sensing, and computing. We use ionic-liquid-assisted ferroelectric switching to demonstrate reversible modulation of interfacial magnetism in a multiferroic heterostructure composed of ferromagnetic (FM) La0.8Sr0.2MnO3 and ferroelectric (FE) PbZr0.2Ti0.8O3. It is shown that ionic liquids can be used to persistently and reversibly switch a large area of a FE film. This is a prerequisite for polarized neutron reflectometry (PNR) studies that are conducted to directly probe magnetoelectric coupling of the FE polarization to the interfacial magnetization.

KW - Magnetoelectric coupling

KW - ferroelectric field effect

KW - ionic liquid gating

KW - polarized neutron reflectometry

KW - strongly correlated oxide

UR - https://www.scopus.com/pages/publications/85014953711

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DO - 10.1021/acs.nanolett.6b04949

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JO - Nano Letters

JF - Nano Letters

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ER -

Reversible Control of Interfacial Magnetism through Ionic-Liquid-Assisted Polarization Switching

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Keywords

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