Resonance in the electron-doped high-transition-temperature superconductor Pr0.88LaCe0.12CuO4-δ

Stephen D. Wilson, Pengcheng Dai, Shiliang Li, Songxue Chi, H. J. Kang, J. W. Lynn

Research output: Contribution to journalArticlepeer-review

109 Scopus citations

Abstract

In conventional superconductors, the interaction that pairs the electrons to form the superconducting state is mediated by lattice vibrations (phonons). In high-transition-temperature (high-Tc) copper oxides, it is generally believed that magnetic excitations might play a fundamental role in the superconducting mechanism because superconductivity occurs when mobile 'electrons' or 'holes' are doped into the antiferromagnetic parent compounds. Indeed, a sharp magnetic excitation termed 'resonance' has been observed by neutron scattering in a number of hole-doped materials. The resonance is intimately related to superconductivity, and its interaction with charged quasi-particles observed by photoemission, optical conductivity, and tunnelling suggests that it might play a part similar to that of phonons in conventional superconductors. The relevance of the resonance to high-Tc superconductivity, however, has been in doubt because so far it has been found only in hole-doped materials. Here we report the discovery of the resonance in electron-doped superconducting Pr0.88LaCe0.12CuO 4-δ (Tc = 24 K). We find that the resonance energy (Er) is proportional to Tc via Er ≈ 5.8kBTc for all high-Tc superconductors irrespective of electron- or hole-doping. Our results demonstrate that the resonance is a fundamental property of the superconducting copper oxides and therefore must be essential in the mechanism of superconductivity.

Original languageEnglish
Pages (from-to)59-62
Number of pages4
JournalNature
Volume442
Issue number7098
DOIs
StatePublished - Jul 6 2006
Externally publishedYes

Funding

Acknowledgements We thank E. Dagotto, H. Ding and S. Zhang for discussions. We also thank Y. Ando’s group for teaching us how to grow high-quality single crystals of PLCCO. S.D.W. and S.L. are supported by the US National Science Foundation. S.C. is supported by the US DOE Division of Materials Science, Basic Energy Sciences. Oak Ridge National Laboratory is supported by the US DOE through UT/Battelle LLC. SPINS is supported by the US National Science Foundation through the Center for High Resolution Neutron Spectroscopy.

FundersFunder number
Center for High Resolution Neutron Spectroscopy
US DOE Division of Materials Science
US National Science Foundation
UT/Battelle LLC
U.S. Department of Energy
Basic Energy Sciences

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