Resonance from antiferromagnetic spin fluctuations for superconductivity in UTe2

Chunruo Duan, R. E. Baumbach, Andrey Podlesnyak, Yuhang Deng, Camilla Moir, Alexander J. Breindel, M. Brian Maple, E. M. Nica, Qimiao Si, Pengcheng Dai

Research output: Contribution to journalArticlepeer-review

49 Scopus citations

Abstract

Superconductivity originates from the formation of bound (Cooper) pairs of electrons that can move through the lattice without resistance below the superconducting transition temperature Tc (ref. 1). Electron Cooper pairs in most superconductors form anti-parallel spin singlets with total spin S = 0 (ref. 2), although they can also form parallel spin-triplet Cooper pairs with S = 1 and an odd parity wavefunction3. Spin-triplet pairing is important because it can host topological states and Majorana fermions relevant for quantum computation4,5. Because spin-triplet pairing is usually mediated by ferromagnetic (FM) spin fluctuations3, uranium-based materials near an FM instability are considered to be ideal candidates for realizing spin-triplet superconductivity6. Indeed, UTe2, which has a Tc ≈ 1.6 K (refs. 7,8), has been identified as a candidate for a chiral spin-triplet topological superconductor near an FM instability7–14, although it also has antiferromagnetic (AF) spin fluctuations15,16. Here we use inelastic neutron scattering (INS) to show that superconductivity in UTe2 is coupled to a sharp magnetic excitation, termed resonance17–23, at the Brillouin zone boundary near AF order. Because the resonance has only been found in spin-singlet unconventional superconductors near an AF instability17–23, its observation in UTe2 suggests that AF spin fluctuations may also induce spin-triplet pairing24 or that electron pairing in UTe2 has a spin-singlet component.

Original languageEnglish
Pages (from-to)636-640
Number of pages5
JournalNature
Volume600
Issue number7890
DOIs
StatePublished - Dec 23 2021

Funding

Acknowledgements P.D. thanks D. Natelson, W. P. Halperin, N. Butch and J. Paglione for discussions. E.M.N. and Q.S. acknowledge discussions with H. Hu, S. Paschen and J.-X. Zhu. The INS work at Rice is supported by the US DOE, BES under grant no. DE-SC0012311 (P.D.). Part of the material characterization efforts at Rice is supported by the Robert A. Welch Foundation grant nos C-1839 (P.D.). Work performed by R.E.B. at the National High Magnetic Field Laboratory was supported by National Science Foundation Cooperative Agreement No. DMR-1644779 and the State of Florida. Synthesis of crystalline materials and measurements by R.E.B. were supported by the Center for Actinide Science and Technology (CAST), an Energy Frontier Research Center (EFRC) funded by the US DOE, BES, under grant no. DE-SC0016568. Research at UC San Diego was supported by the US DOE, BES under grant no. DEFG02-04-ER46105 (single-crystal growth) and US NSF under grant no. DMR-1810310 (characterization of physical properties). The theory work at Rice has primarily been supported by the US DOE, BES under award no. DE-SC0018197, with travel support provided by the Robert A. Welch Foundation grant no. C-1411. Q.S. acknowledges the hospitality of the Aspen Center for Physics, which is supported by NSF grant no. PHY-1607611. E.M.N. was supported by an ASU startup grant. A portion of this research used resources at the Spallation Neutron Source, a DOE Office of Science User Facility operated by ORNL.

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