Removing hydrogen sulfide from hydrogen-rich gas streams by selective catalytic oxidation

Xianxian Wu; Andrew K. Kercher; Viviane Schwartz; Steven H. Overbury; Timothy R. Armstrong

Removing hydrogen sulfide from hydrogen-rich gas streams by selective catalytic oxidation

Xianxian Wu, Andrew K. Kercher, Viviane Schwartz, Steven H. Overbury, Timothy R. Armstrong

Particle Fuel Forms

Research output: Contribution to journal › Conference article › peer-review

3 Scopus citations

Abstract

As the ideal fuel for proton-exchange membrane fuel cells, hydrogen will mainly be generated from fossil fuels by steam reforming or partial oxidation before a long term energy solution is developed. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H₂S in reformate. Test results of an activated carbon made at ORNL were presented, and compared with those of selected commercial carbons using reformate as the model gas stream. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H₂S in reformate. The activated carbon synthesized at ORNL has the ability to selectively oxidize H₂S down to parts per billion level without detectable occurrence of unwanted side-reactions.

Original language	English
Pages (from-to)	893-894
Number of pages	2
Journal	ACS Division of Fuel Chemistry, Preprints
Volume	49
Issue number	2
State	Published - Sep 2004

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title = "Removing hydrogen sulfide from hydrogen-rich gas streams by selective catalytic oxidation",

abstract = "As the ideal fuel for proton-exchange membrane fuel cells, hydrogen will mainly be generated from fossil fuels by steam reforming or partial oxidation before a long term energy solution is developed. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H2S in reformate. Test results of an activated carbon made at ORNL were presented, and compared with those of selected commercial carbons using reformate as the model gas stream. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H2S in reformate. The activated carbon synthesized at ORNL has the ability to selectively oxidize H2S down to parts per billion level without detectable occurrence of unwanted side-reactions.",

author = "Xianxian Wu and Kercher, {Andrew K.} and Viviane Schwartz and Overbury, {Steven H.} and Armstrong, {Timothy R.}",

year = "2004",

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journal = "ACS Division of Fuel Chemistry, Preprints",

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T1 - Removing hydrogen sulfide from hydrogen-rich gas streams by selective catalytic oxidation

AU - Wu, Xianxian

AU - Kercher, Andrew K.

AU - Schwartz, Viviane

AU - Overbury, Steven H.

AU - Armstrong, Timothy R.

PY - 2004/9

Y1 - 2004/9

N2 - As the ideal fuel for proton-exchange membrane fuel cells, hydrogen will mainly be generated from fossil fuels by steam reforming or partial oxidation before a long term energy solution is developed. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H2S in reformate. Test results of an activated carbon made at ORNL were presented, and compared with those of selected commercial carbons using reformate as the model gas stream. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H2S in reformate. The activated carbon synthesized at ORNL has the ability to selectively oxidize H2S down to parts per billion level without detectable occurrence of unwanted side-reactions.

AB - As the ideal fuel for proton-exchange membrane fuel cells, hydrogen will mainly be generated from fossil fuels by steam reforming or partial oxidation before a long term energy solution is developed. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H2S in reformate. Test results of an activated carbon made at ORNL were presented, and compared with those of selected commercial carbons using reformate as the model gas stream. The formation of COS is a problem for the use of commercial activated carbons as the oxidation catalysts of H2S in reformate. The activated carbon synthesized at ORNL has the ability to selectively oxidize H2S down to parts per billion level without detectable occurrence of unwanted side-reactions.

UR - http://www.scopus.com/inward/record.url?scp=4544262909&partnerID=8YFLogxK

M3 - Conference article

AN - SCOPUS:4544262909

SN - 0569-3772

VL - 49

SP - 893

EP - 894

JO - ACS Division of Fuel Chemistry, Preprints

JF - ACS Division of Fuel Chemistry, Preprints

IS - 2

ER -

Removing hydrogen sulfide from hydrogen-rich gas streams by selective catalytic oxidation

Abstract

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