Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells

Andrew J. Steinbach; Dennis Van Der Vliet; Amy E. Hester; Jonah Erlebacher; Cemal Duru; Isaac Davy; Monika Kuznia; David A. Cullen

doi:10.1149/06917.0291ecst

Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells

Andrew J. Steinbach, Dennis Van Der Vliet, Amy E. Hester, Jonah Erlebacher, Cemal Duru, Isaac Davy, Monika Kuznia, David A. Cullen

Materials MicroAnalysis

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

5 Scopus citations

Abstract

In this paper, we provide an overview of several recent development activities towards improving the activity of nanoporous Pt_xNi_1-x thin film electrocatalysts on the 3M Nanostructured Thin Film (NSTF) support. Significant improvements in electrocatalyst specific area and mass activity have been achieved through optimization of electrocatalyst fabrication parameters (deposition, annealing, and dealloying), which influence electrocatalyst composition and structure. Membrane electrode assemblies (MEAs) which incorporate improved NSTF Pt_xNi_1-x cathode catalysts have demonstrated performances which approach or exceed several U.S. Department of Energy 2020 performance and PGM-content targets.

Original language	English
Title of host publication	Polymer Electrolyte Fuel Cells 15, PEFC 15
Editors	H. A. Gasteiger, A. Z. Weber, V. K. Ramani, T. F. Fuller, R. A. Mantz, H. Uchida, F. N. Buchi, M. Edmundson, C. Coutanceau, J. M. Fenton, S. Mitsushima, T. J. Schmidt, K. Shinohara, K. Swider-Lyons, D. J. Jones, B. S. Pivovar, K. E. Ayers, K. A. Perry, S. R. Narayanan, P. Strasser
Publisher	Electrochemical Society Inc.
Pages	291-301
Number of pages	11
Edition	17
ISBN (Electronic)	9781607685395
DOIs	https://doi.org/10.1149/06917.0291ecst
State	Published - 2015
Event	Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting - Phoenix, United States Duration: Oct 11 2015 → Oct 15 2015

Publication series

Name	ECS Transactions
Number	17
Volume	69
ISSN (Print)	1938-6737
ISSN (Electronic)	1938-5862

Conference

Conference	Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting
Country/Territory	United States
City	Phoenix
Period	10/11/15 → 10/15/15

Bibliographical note

Publisher Copyright:
© The Electrochemical Society.

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Steinbach, A. J., Van Der Vliet, D., Hester, A. E., Erlebacher, J., Duru, C., Davy, I., Kuznia, M., & Cullen, D. A. (2015). Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells. In H. A. Gasteiger, A. Z. Weber, V. K. Ramani, T. F. Fuller, R. A. Mantz, H. Uchida, F. N. Buchi, M. Edmundson, C. Coutanceau, J. M. Fenton, S. Mitsushima, T. J. Schmidt, K. Shinohara, K. Swider-Lyons, D. J. Jones, B. S. Pivovar, K. E. Ayers, K. A. Perry, S. R. Narayanan, & P. Strasser (Eds.), Polymer Electrolyte Fuel Cells 15, PEFC 15 (17 ed., pp. 291-301). (ECS Transactions; Vol. 69, No. 17). Electrochemical Society Inc.. https://doi.org/10.1149/06917.0291ecst

Steinbach, Andrew J. ; Van Der Vliet, Dennis ; Hester, Amy E. et al. / Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells. Polymer Electrolyte Fuel Cells 15, PEFC 15. editor / H. A. Gasteiger ; A. Z. Weber ; V. K. Ramani ; T. F. Fuller ; R. A. Mantz ; H. Uchida ; F. N. Buchi ; M. Edmundson ; C. Coutanceau ; J. M. Fenton ; S. Mitsushima ; T. J. Schmidt ; K. Shinohara ; K. Swider-Lyons ; D. J. Jones ; B. S. Pivovar ; K. E. Ayers ; K. A. Perry ; S. R. Narayanan ; P. Strasser. 17. ed. Electrochemical Society Inc., 2015. pp. 291-301 (ECS Transactions; 17).

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title = "Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells",

abstract = "In this paper, we provide an overview of several recent development activities towards improving the activity of nanoporous PtxNi1-x thin film electrocatalysts on the 3M Nanostructured Thin Film (NSTF) support. Significant improvements in electrocatalyst specific area and mass activity have been achieved through optimization of electrocatalyst fabrication parameters (deposition, annealing, and dealloying), which influence electrocatalyst composition and structure. Membrane electrode assemblies (MEAs) which incorporate improved NSTF PtxNi1-x cathode catalysts have demonstrated performances which approach or exceed several U.S. Department of Energy 2020 performance and PGM-content targets.",

author = "Steinbach, {Andrew J.} and {Van Der Vliet}, Dennis and Hester, {Amy E.} and Jonah Erlebacher and Cemal Duru and Isaac Davy and Monika Kuznia and Cullen, {David A.}",

note = "Publisher Copyright: {\textcopyright} The Electrochemical Society.; Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting ; Conference date: 11-10-2015 Through 15-10-2015",

year = "2015",

doi = "10.1149/06917.0291ecst",

language = "English",

series = "ECS Transactions",

publisher = "Electrochemical Society Inc.",

number = "17",

pages = "291--301",

editor = "Gasteiger, {H. A.} and Weber, {A. Z.} and Ramani, {V. K.} and Fuller, {T. F.} and Mantz, {R. A.} and H. Uchida and Buchi, {F. N.} and M. Edmundson and C. Coutanceau and Fenton, {J. M.} and S. Mitsushima and Schmidt, {T. J.} and K. Shinohara and K. Swider-Lyons and Jones, {D. J.} and Pivovar, {B. S.} and Ayers, {K. E.} and Perry, {K. A.} and Narayanan, {S. R.} and P. Strasser",

booktitle = "Polymer Electrolyte Fuel Cells 15, PEFC 15",

edition = "17",

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Steinbach, AJ, Van Der Vliet, D, Hester, AE, Erlebacher, J, Duru, C, Davy, I, Kuznia, M & Cullen, DA 2015, Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells. in HA Gasteiger, AZ Weber, VK Ramani, TF Fuller, RA Mantz, H Uchida, FN Buchi, M Edmundson, C Coutanceau, JM Fenton, S Mitsushima, TJ Schmidt, K Shinohara, K Swider-Lyons, DJ Jones, BS Pivovar, KE Ayers, KA Perry, SR Narayanan & P Strasser (eds), Polymer Electrolyte Fuel Cells 15, PEFC 15. 17 edn, ECS Transactions, no. 17, vol. 69, Electrochemical Society Inc., pp. 291-301, Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting, Phoenix, United States, 10/11/15. https://doi.org/10.1149/06917.0291ecst

Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells. / Steinbach, Andrew J.; Van Der Vliet, Dennis; Hester, Amy E. et al.
Polymer Electrolyte Fuel Cells 15, PEFC 15. ed. / H. A. Gasteiger; A. Z. Weber; V. K. Ramani; T. F. Fuller; R. A. Mantz; H. Uchida; F. N. Buchi; M. Edmundson; C. Coutanceau; J. M. Fenton; S. Mitsushima; T. J. Schmidt; K. Shinohara; K. Swider-Lyons; D. J. Jones; B. S. Pivovar; K. E. Ayers; K. A. Perry; S. R. Narayanan; P. Strasser. 17. ed. Electrochemical Society Inc., 2015. p. 291-301 (ECS Transactions; Vol. 69, No. 17).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

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T1 - Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells

AU - Steinbach, Andrew J.

AU - Van Der Vliet, Dennis

AU - Hester, Amy E.

AU - Erlebacher, Jonah

AU - Duru, Cemal

AU - Davy, Isaac

AU - Kuznia, Monika

AU - Cullen, David A.

N1 - Publisher Copyright: © The Electrochemical Society.

PY - 2015

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N2 - In this paper, we provide an overview of several recent development activities towards improving the activity of nanoporous PtxNi1-x thin film electrocatalysts on the 3M Nanostructured Thin Film (NSTF) support. Significant improvements in electrocatalyst specific area and mass activity have been achieved through optimization of electrocatalyst fabrication parameters (deposition, annealing, and dealloying), which influence electrocatalyst composition and structure. Membrane electrode assemblies (MEAs) which incorporate improved NSTF PtxNi1-x cathode catalysts have demonstrated performances which approach or exceed several U.S. Department of Energy 2020 performance and PGM-content targets.

AB - In this paper, we provide an overview of several recent development activities towards improving the activity of nanoporous PtxNi1-x thin film electrocatalysts on the 3M Nanostructured Thin Film (NSTF) support. Significant improvements in electrocatalyst specific area and mass activity have been achieved through optimization of electrocatalyst fabrication parameters (deposition, annealing, and dealloying), which influence electrocatalyst composition and structure. Membrane electrode assemblies (MEAs) which incorporate improved NSTF PtxNi1-x cathode catalysts have demonstrated performances which approach or exceed several U.S. Department of Energy 2020 performance and PGM-content targets.

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SP - 291

EP - 301

BT - Polymer Electrolyte Fuel Cells 15, PEFC 15

A2 - Gasteiger, H. A.

A2 - Weber, A. Z.

A2 - Ramani, V. K.

A2 - Fuller, T. F.

A2 - Mantz, R. A.

A2 - Uchida, H.

A2 - Buchi, F. N.

A2 - Edmundson, M.

A2 - Coutanceau, C.

A2 - Fenton, J. M.

A2 - Mitsushima, S.

A2 - Schmidt, T. J.

A2 - Shinohara, K.

A2 - Swider-Lyons, K.

A2 - Jones, D. J.

A2 - Pivovar, B. S.

A2 - Ayers, K. E.

A2 - Perry, K. A.

A2 - Narayanan, S. R.

A2 - Strasser, P.

PB - Electrochemical Society Inc.

T2 - Symposium on Polymer Electrolyte Fuel Cells 15, PEFC 2015 - 228th ECS Meeting

Y2 - 11 October 2015 through 15 October 2015

ER -

Steinbach AJ, Van Der Vliet D, Hester AE, Erlebacher J, Duru C, Davy I et al. Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells. In Gasteiger HA, Weber AZ, Ramani VK, Fuller TF, Mantz RA, Uchida H, Buchi FN, Edmundson M, Coutanceau C, Fenton JM, Mitsushima S, Schmidt TJ, Shinohara K, Swider-Lyons K, Jones DJ, Pivovar BS, Ayers KE, Perry KA, Narayanan SR, Strasser P, editors, Polymer Electrolyte Fuel Cells 15, PEFC 15. 17 ed. Electrochemical Society Inc. 2015. p. 291-301. (ECS Transactions; 17). doi: 10.1149/06917.0291ecst

Recent progress in Nanostructured Thin Film (NSTF) ORR electrocatalyst development for PEM fuel cells

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