Quantum-well photoemission spectroscopy of atomically-uniform films

T. Miller, J. J. Paggel, D. A. Luh, T. C. Chiang

Research output: Contribution to journalConference articlepeer-review

7 Scopus citations

Abstract

Using a low-temperature growth technique and an Fe whisker sample, atomically-uniform films of Ag on Fe(100) are prepared. Extremely sharp quantum-well peaks are obtained in these films, as peak broadening from thickness variation is eliminated. The quality of the spectra allows the observation of quantum-well peaks in films over 100 monolayers thick. Quantum-well peaks from both the sp and d states have been observed and used to map the associated bands. The elimination of broadening from thickness variation allows for the interpretation of the peak linewidths in terms of the quasiparticle lifetime and interfacial reflectivity, and the phonon contribution can be deduced from the temperature dependence of the spectra.

Original languageEnglish
Pages (from-to)513-519
Number of pages7
JournalJournal of Electron Spectroscopy and Related Phenomena
Volume114-116
DOIs
StatePublished - Mar 2001
Externally publishedYes
Event8th International Conference on Electronic Spectroscopy and Structure (ICESS-8) - Berkeley, CA, USA
Duration: Aug 8 2000Aug 12 2000

Funding

This material is based upon work supported by the US National Science Foundation, under Grant Nos. DMR-99-75182 and 99-75470. An acknowledgement is made to the Donors of the Petroleum Research Fund, administered by the American Chemical Society, and to the US Department of Energy, Division of Materials Sciences, (Grant No. DEFG02-91ER45439) for partial support of the synchrotron beamline operation and for support of the central facilities of the Materials Research Laboratory. The Synchrotron Radiation Center of the University of Wisconsin is supported by the National Science Foundation under Grant No. DMR-95-31009.

FundersFunder number
Division of Materials SciencesDEFG02-91ER45439
National Science Foundation99-75470, DMR-99-75182, DMR-95-31009
U.S. Department of Energy
American Chemical Society

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