Quantum critical behavior in the asymptotic limit of high disorder in the medium entropy alloy NiCoCr0.8

Brian C. Sales, Ke Jin, Hongbin Bei, John Nichols, Matthew F. Chisholm, Andrew F. May, Nicholas P. Butch, Andrew D. Christianson, Michael A. McGuire

Research output: Contribution to journalArticlepeer-review

23 Scopus citations

Abstract

The behavior of matter near a quantum critical point is one of the most exciting and challenging areas of physics research. Emergent phenomena such as high-temperature superconductivity are linked to the proximity to a quantum critical point. Although significant progress has been made in understanding quantum critical behavior in some low dimensional magnetic insulators, the situation in metallic systems is much less clear. Here, we demonstrate that NiCoCrx single crystal alloys are remarkable model systems for investigating quantum critical point physics in a metallic environment. For NiCoCrx alloys with x ≈ 0.8, the critical exponents associated with a ferromagnetic quantum critical point are experimentally determined from low temperature magnetization and heat capacity measurements. All of the five exponents (γ T ≈ 1/2, β T ≈ 1, δ ≈ 3/2, νzm ≈ 2, α α T ≈ 0) are in remarkable agreement with predictions of Belitz-Kirkpatrick-Vojta theory in the asymptotic limit of high disorder. Using these critical exponents, excellent scaling of the magnetization data is demonstrated with no adjustable parameters. We also find a divergence of the magnetic Gruneisen parameter, consistent with a ferromagnetic quantum critical point. This work therefore demonstrates that entropy stabilized concentrated solid solutions represent a unique platform to study quantum critical behavior in a highly tunable class of materials.

Original languageEnglish
Article number33
Journalnpj Quantum Materials
Volume2
Issue number1
DOIs
StatePublished - Dec 1 2017

Funding

It is a pleasure to acknowledge helpful discussions with Jamie Morris, Lekh Poudel, Malcolm Stocks, German Samolyuk, Claudia Troparevsky and Jiaqiang Yan. I particularly want to thank Claudia Troparevsky for providing an extensive list of predicted ternary solid solution alloys using the methodology developed in reference15. This research was supported primarily by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division (B.C.S., J.N., A.F.M., M.F.C., M.A.M.). K.J. and H.B. were supported by the Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U. S. Department of Energy, Office of Science, BES. Research at ORNL’s Spallation Neutron Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U S. Department of Energy (A.C.).

FundersFunder number
Office of Basic Energy Sciences
Scientific User Facilities Division
U S. Department of Energy
U. S. Department of Energy
U.S. Department of Energy
Office of Science
Basic Energy Sciences
Division of Materials Sciences and Engineering

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