Pressure-induced double superconducting domes and charge instability in the kagome metal KV3Sb5

Feng Du, Shuaishuai Luo, Brenden R. Ortiz, Ye Chen, Weiyin Duan, Dongting Zhang, Xin Lu, Stephen D. Wilson, Yu Song, Huiqiu Yuan

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129 Scopus citations

Abstract

The kagome metal KV3Sb5 hosts charge order, topologically nontrivial Dirac band crossings, and a superconducting ground state with unconventional characteristics, providing an ideal platform to investigate the interplay between different electronic states on the kagome lattice. Here we study the evolution of charge order and superconductivity in KV3Sb5 under hydrostatic pressure using electrical resistivity measurements. With the application of pressure, the superconducting transition temperature Tc=0.9 K under ambient pressure quickly increases to 3.1 K at p=0.4 GPa, as charge order progressively weakens. Upon further increasing pressure, signatures of charge order disappear at pc1≈0.5 GPa and Tc is gradually suppressed, forming a superconducting dome that terminates at p≈10 GPa. Beyond p≈10 GPa, a second superconducting dome emerges with maximum Tc≈1.0 K at pc2≈22 GPa, which becomes fully suppressed at p≈28 GPa. The suppression of superconductivity for the second superconducting dome is associated with the appearance of a unique high-pressure phase, possibly a distinct charge order.

Original languageEnglish
Article numberL220504
JournalPhysical Review B
Volume103
Issue number22
DOIs
StatePublished - Jun 1 2021
Externally publishedYes

Funding

This work was supported by the National Key R&D Program of China (Grants No. 2017YFA0303100 and No. 2016YFA0300202), the Key R&D Program of Zhejiang Province, China (Grant No. 2021C01002), the National Natural Science Foundation of China (Grants No. 11974306 and No. 12034017), the Science Challenge Project of China (Grant No. TZ2016004), and the Fundamental Research Funds for the Central Universities of China. S.D.W. and B.R.O. gratefully acknowledge support via the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under Award No. DMR-1906325. B.R.O. also acknowledges support from the California NanoSystems Institute through the Elings fellowship program.

FundersFunder number
California NanoSystems Institute
Key R&D Program of Zhejiang Province2021C01002
Science Challenge Project of ChinaTZ2016004
UC Santa Barbara NSFDMR-1906325
National Natural Science Foundation of China12034017, 11974306
National Key Research and Development Program of China2017YFA0303100, 2016YFA0300202
Fundamental Research Funds for the Central Universities

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