Abstract
Since the earliest investigations of olefin metathesis catalysis, light has been the choice for controlling the catalyst activity on demand. From the perspective of energy efficiency, temporal and spatial control, and selectivity, photochemistry is not only an attractive alternative to traditional thermal manufacturing techniques but also arguably a superior manifold for advanced applications like additive manufacturing (AM). In the last three decades, pioneering work in the field of ring-opening metathesis polymerization (ROMP) has broadened the scope of material properties achievable through AM, particularly using light as both an activating and deactivating stimulus. In this Perspective, we explore trends in photocontrolled ROMP systems with an emphasis on approaches to photoinduced activation and deactivation of metathesis catalysts. Recent work has yielded a myriad of commercial and synthetically accessible photosensitive catalyst systems, although comparatively little attention has been paid to achieving precise control over polymer morphology using light. Metal-free, photophysical, and living ROMP systems have also been relatively underexplored. To take fuller advantage of both the thermomechanical properties of ROMP polymers and the operational simplicity of photocontrol, clear directions for the field are to improve the reversibility of activation and deactivation strategies as well as to further develop photocontrolled approaches to tuning cross-link density and polymer tacticity.
Original language | English |
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Pages (from-to) | 6217-6227 |
Number of pages | 11 |
Journal | ACS Catalysis |
Volume | 14 |
Issue number | 8 |
DOIs | |
State | Published - Apr 19 2024 |
Funding
The authors thank Leah Appelhans for their review of this manuscript. This paper describes objective technical results and analysis. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, a multimission laboratory managed and operated by the National Technology and Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International, Inc., for the U.S. Department of Energy\u2019s National Nuclear Security Administration under contract DE-NA-0003525. This work was also sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory managed by UT-Battelle LLC for the U.S. DOE.
Keywords
- olefin metathesis
- photocatalysis
- photocontrol
- ring-opening metathesis
- ruthenium