Photon correlation spectroscopy of colloidal palladium using a coherent x-ray beam

T. Thurn-Albrecht; W. Steffen; A. Patkowski; G. Meier; E. W. Fischer; G. Grübel; D. L. Abernathy

doi:10.1103/PhysRevLett.77.5437

Photon correlation spectroscopy of colloidal palladium using a coherent x-ray beam

T. Thurn-Albrecht, W. Steffen, A. Patkowski, G. Meier, E. W. Fischer, G. Grübel, D. L. Abernathy

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106 Scopus citations

Abstract

We have used an intense coherent x-ray beam and a real time digital autocorrelator to study the low frequency dynamics of colloidal palladium in glycerol by x-ray photon correlation spectroscopy (XPCS). The translational diffusion was studied in the q range from 1.5 × 10⁻³ to 6 × 10⁻³Å⁻¹ and in the temperature range from 279 to 293K. The measured relaxation rates were proportional to q² and inversely proportional to viscosity as expected for a translational diffusion process. This experiment shows that XPCS can be performed in a wide time range (10⁻⁴ to 100s) and opens up a new opportunity for the study of the dynamics of nontransparent media.

Original language	English
Pages (from-to)	5437-5440
Number of pages	4
Journal	Physical Review Letters
Volume	77
Issue number	27
DOIs	https://doi.org/10.1103/PhysRevLett.77.5437
State	Published - 1996
Externally published	Yes

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title = "Photon correlation spectroscopy of colloidal palladium using a coherent x-ray beam",

abstract = "We have used an intense coherent x-ray beam and a real time digital autocorrelator to study the low frequency dynamics of colloidal palladium in glycerol by x-ray photon correlation spectroscopy (XPCS). The translational diffusion was studied in the q range from 1.5 × 10−3 to 6 × 10−3{\AA}−1 and in the temperature range from 279 to 293K. The measured relaxation rates were proportional to q2 and inversely proportional to viscosity as expected for a translational diffusion process. This experiment shows that XPCS can be performed in a wide time range (10−4 to 100s) and opens up a new opportunity for the study of the dynamics of nontransparent media.",

author = "T. Thurn-Albrecht and W. Steffen and A. Patkowski and G. Meier and Fischer, \{E. W.\} and G. Gr{\"u}bel and Abernathy, \{D. L.\}",

year = "1996",

doi = "10.1103/PhysRevLett.77.5437",

language = "English",

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journal = "Physical Review Letters",

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T1 - Photon correlation spectroscopy of colloidal palladium using a coherent x-ray beam

AU - Thurn-Albrecht, T.

AU - Steffen, W.

AU - Patkowski, A.

AU - Meier, G.

AU - Fischer, E. W.

AU - Grübel, G.

AU - Abernathy, D. L.

PY - 1996

Y1 - 1996

N2 - We have used an intense coherent x-ray beam and a real time digital autocorrelator to study the low frequency dynamics of colloidal palladium in glycerol by x-ray photon correlation spectroscopy (XPCS). The translational diffusion was studied in the q range from 1.5 × 10−3 to 6 × 10−3Å−1 and in the temperature range from 279 to 293K. The measured relaxation rates were proportional to q2 and inversely proportional to viscosity as expected for a translational diffusion process. This experiment shows that XPCS can be performed in a wide time range (10−4 to 100s) and opens up a new opportunity for the study of the dynamics of nontransparent media.

AB - We have used an intense coherent x-ray beam and a real time digital autocorrelator to study the low frequency dynamics of colloidal palladium in glycerol by x-ray photon correlation spectroscopy (XPCS). The translational diffusion was studied in the q range from 1.5 × 10−3 to 6 × 10−3Å−1 and in the temperature range from 279 to 293K. The measured relaxation rates were proportional to q2 and inversely proportional to viscosity as expected for a translational diffusion process. This experiment shows that XPCS can be performed in a wide time range (10−4 to 100s) and opens up a new opportunity for the study of the dynamics of nontransparent media.

UR - https://www.scopus.com/pages/publications/0030391907

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DO - 10.1103/PhysRevLett.77.5437

M3 - Article

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SN - 0031-9007

VL - 77

SP - 5437

EP - 5440

JO - Physical Review Letters

JF - Physical Review Letters

IS - 27

ER -

Photon correlation spectroscopy of colloidal palladium using a coherent x-ray beam

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