Persistence of local-moment antiferromagnetic order in Ba 1-xKxMn2As2

J. Lamsal, G. S. Tucker, T. W. Heitmann, A. Kreyssig, A. Jesche, Abhishek Pandey, Wei Tian, R. J. McQueeney, D. C. Johnston, A. I. Goldman

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Abstract

BaMn2As2 is a local-moment antiferromagnetic insulator with a Néel temperature TN of 625 K and a large ordered moment of 3.9 μB/Mn. Remarkably, this compound can be driven metallic by the substitution of as little as 1.6% K for Ba while retaining essentially the same ordered magnetic moment and Néel temperature, as previously reported. Here, using both powder and single crystal neutron diffraction we show that the local moment antiferromagnetic order in Ba1-xKxMn2As2 remains robust up to x=0.4. The ordered moment is nearly independent of x for 0 ≤x≤ 0.4 and TN decreases to 480 K at x=0.4.

Original languageEnglish
Article number144418
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume87
Issue number14
DOIs
StatePublished - Apr 24 2013

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