Oval-cycloidal magnetic structure with phase-shift in the non-centrosymmetric tetragonal compound CePdSi3

Daichi Ueta, Masahiro Yoshida, Tomohiro Kobuke, Yoichi Ikeda, Akiko Nakao, Taketo Moyoshi, Koji Munakata, Yaohua Liu, Takatsugu Masuda, Hideki Yoshizawa

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    Abstract

    CePdSi3 with H == [100] exhibits multiple metamagnetic transitions. Since there is no frustration in this system, it is suggested that the origin of the multiple metamagnetic transitions is the influence of the antisymmetric spin-orbit interaction. To clarify the magnetic structure under the influence of the antisymmetric spin-orbit interaction, neutron diffraction experiments have been performed using single crystal samples of CePdSi3. There are observed magnetic reflections with incommensurate magnetic propagation vector q ¼ ð0:315; 0; 0Þ in the phase I. In addition, additional magnetic reflections were also observed in the phase III. The magnetic structure was found to be an oval-cycloidal structure at the phase III in CePdSi3, and we discuss the origin of the unusual magnetic structure.

    Original languageEnglish
    Article number114702
    JournalJournal of the Physical Society of Japan
    Volume90
    Issue number11
    DOIs
    StatePublished - Nov 15 2021

    Funding

    This research used resources at the Spallation Neutron Source (SNS), a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory (ORNL), and resources of the SNS Second Target Station Project. ORNL is managed by UT-Battelle LLC for DOE's Office of Science, the single largest supporter of basic research in the physical sciences in the United States. The neutron diffraction experiments performed on CORELLI at SNS, ORNL, USA was supported by the General User Program for Neutron Scattering Experiments, Institute for Solid State Physics, The University of Tokyo (Proposal No. 17507). The neutron diffraction measurements on SENJU at J-PARC, MLF was performed as a general proposal of MLF=J-PARC (Nos. 2017A0223, 2017B0098). We thank the preparation of the refrigeration system to perform these experiments. One of the authors D.U. would like to thank Professor T. Arima, Professor K. Iwasa, and Dr. S. Asai for valuable comments and discussions. This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). Acknowledgment This research used resources at the Spallation Neutron Source (SNS), a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory (ORNL), and resources of the SNS Second Target Station Project. ORNL is managed by UT-Battelle LLC for DOE\u2019s Office of Science, the single largest supporter of basic research in the physical sciences in the United States. The neutron diffraction experiments performed on CORELLI at SNS, ORNL, USA was supported by the General User Program for Neutron Scattering Experiments, Institute for Solid State Physics, The University of Tokyo (Proposal No. 17507). The neutron diffraction measurements on SENJU at J-PARC, MLF was performed as a general proposal of MLF=J-PARC (Nos. 2017A0223, 2017B0098). We thank the preparation of the refrigeration system to perform these experiments. One of the authors D.U. would like to thank Professor T. Arima, Professor K. Iwasa, and Dr. S. Asai for valuable comments and discussions. This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/ doe-public-access-plan).

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