One-step synthesis of nitrogen-doped graphene-like meso-macroporous carbons as highly efficient and selective adsorbents for CO2 capture

Fujian Liu; Kuan Huang; Shunmin Ding; Sheng Dai

doi:10.1039/c6ta06583j

One-step synthesis of nitrogen-doped graphene-like meso-macroporous carbons as highly efficient and selective adsorbents for CO₂ capture

Fujian Liu, Kuan Huang, Shunmin Ding, Sheng Dai

Chemical Sciences Division

Research output: Contribution to journal › Article › peer-review

72 Scopus citations

Abstract

Graphene-like meso-macroporous carbons (GMCs) with high nitrogen contents and controllable nitrogen sites were synthesized by one-step carbonization of dicyandiamide or melamine with glucose. The unique layered structure and the presence of abundant meso-macropores in GMCs largely enhance the degree of exposure and accessibility of anchored nitrogen sites to CO₂, which provides the GMCs with excellent performance for the selective capture of CO₂.

Original language	English
Pages (from-to)	14567-14571
Number of pages	5
Journal	Journal of Materials Chemistry A
Volume	4
Issue number	38
DOIs	https://doi.org/10.1039/c6ta06583j
State	Published - 2016

Funding

This work was supported as part of the Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0012577. F. L. acknowledges the financial support of the National Natural Science Foundation of China (21573150, 21203122) and the Natural Science Foundation of Zhejiang Province (LY15B030002)

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1039/c6ta06583j

Cite this

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