TY - JOUR
T1 - Observation of Magnetoelectric Multiferroicity in a Cubic Perovskite System
T2 - LaMn3Cr4O12
AU - Wang, Xiao
AU - Chai, Yisheng
AU - Zhou, Long
AU - Cao, Huibo
AU - Cruz, Clarina Dela
AU - Yang, Junye
AU - Dai, Jianhong
AU - Yin, Yunyu
AU - Yuan, Zhen
AU - Zhang, Sijia
AU - Yu, Runze
AU - Azuma, Masaki
AU - Shimakawa, Yuichi
AU - Zhang, Huimin
AU - Dong, Shuai
AU - Sun, Young
AU - Jin, Changqing
AU - Long, Youwen
N1 - Publisher Copyright:
© 2015 American Physical Society.
PY - 2015/8/18
Y1 - 2015/8/18
N2 - Magnetoelectric multiferroicity is not expected to occur in a cubic perovskite system because of the high structural symmetry. By versatile measurements in magnetization, dielectric constant, electric polarization, neutron and x-ray diffraction, Raman scattering, as well as theoretical calculations, we reveal that the A-site ordered perovskite LaMn3Cr4O12 with cubic symmetry is a novel spin-driven multiferroic system with strong magnetoelectric coupling effects. When a magnetic field is applied in parallel (perpendicular) to an electric field, the ferroelectric polarization can be enhanced (suppressed) significantly. The unique multiferroic phenomenon observed in this cubic perovskite cannot be understood by conventional spin-driven microscopic mechanisms. Instead, a nontrivial effect involving the interactions between two magnetic sublattices is likely to play a crucial role.
AB - Magnetoelectric multiferroicity is not expected to occur in a cubic perovskite system because of the high structural symmetry. By versatile measurements in magnetization, dielectric constant, electric polarization, neutron and x-ray diffraction, Raman scattering, as well as theoretical calculations, we reveal that the A-site ordered perovskite LaMn3Cr4O12 with cubic symmetry is a novel spin-driven multiferroic system with strong magnetoelectric coupling effects. When a magnetic field is applied in parallel (perpendicular) to an electric field, the ferroelectric polarization can be enhanced (suppressed) significantly. The unique multiferroic phenomenon observed in this cubic perovskite cannot be understood by conventional spin-driven microscopic mechanisms. Instead, a nontrivial effect involving the interactions between two magnetic sublattices is likely to play a crucial role.
UR - http://www.scopus.com/inward/record.url?scp=84940703299&partnerID=8YFLogxK
U2 - 10.1103/PhysRevLett.115.087601
DO - 10.1103/PhysRevLett.115.087601
M3 - Article
AN - SCOPUS:84940703299
SN - 0031-9007
VL - 115
JO - Physical Review Letters
JF - Physical Review Letters
IS - 8
M1 - 087601
ER -