Abstract
The interplay among topology, crystal symmetry, magnetic order, and strong electron correlation can give rise to a plethora of exotic physical phenomena. The ZrSiS family is known as typical topological Dirac semimetals, among them LnSbTe (Ln denotes lanthanide) compounds exhibit intriguing characteristics due to the presence of Ln 4f electrons, resulting in quantum states and unique properties. In this paper, the topological electronic structure of PrSbTe is systematically studied by angle-resolved photoemission spectroscopy (ARPES), combined with magnetic, specific heat measurements, and band structure calculations. The detailed three-dimensional electronic structure of PrSbTe has been obtained, and a diamond-shaped Fermi surface and multiple Dirac nodal lines have been observed, which are in remarkable agreement with theoretical calculations. Moreover, the 4f electrons in PrSbTe are rather localized, which can be revealed by on-resonant ARPES data and further confirmed by the rather small Sommerfeld coefficient of γ=2.6231mJ/molK2. Our results provide more detailed information about the LnSbTe family, which gives a deeper understanding of the interaction between Ln 4f electrons and the topological states.
| Original language | English |
|---|---|
| Article number | 045113 |
| Journal | Physical Review B |
| Volume | 109 |
| Issue number | 4 |
| DOIs | |
| State | Published - Jan 15 2024 |
| Externally published | Yes |
Funding
This paper was supported by the National Key Research and Development Program of China (Grants No. 2022YFA1402201 and No. 2021YFA1601101), the National Science Foundation of China (Grants No. 12122409, No. 11974319, and No. 11904335), the Fund of Science and Technology on Surface Physics and Chemistry Laboratory (No. XKFZ202106), and the Special Talent Fund of the Institute of Materials (No. TP03201901). ARPES measurements were performed in the ARPES endstation of BL03U and BL09U of SSRF, China. The magnetic and specific heat measurements were performed in the Synergetic Extreme Condition User Facility.