Numerical simulation of polymer phase separation on a patterned substrate with nano features

Yingrui Shang, David Kazmer, Ming Wei, Joey Mead, Carol Barry

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

Abstract

Phase separation of an asymmetric immiscible binary polymer system in an elastic field with the existence of a patterned substrate was numerically studied in 2D and 3D. An unconditionally stable method for time marching the Cahn-Hilliard equation was employed in the numerical simulation. Compared to the conventional interface tracing mechanism, this diffusion controlled system is characterized by a thick interface with a composition gradient. The evolution mechanisms were studied. The evolution of the characteristic length, R(t), of the phase separation morphology patterns was measured with the Fast Fourier Transform method. The results indicated R(t)1/3 increases linearly with time. The influence of the material composition, the attraction factor on the template, and the gradient energy coefficient between the two polymers on the result patterns were also observed in this study. Qualitative and quantitative correspondence can be observed between the numerical results and the experiment results.

Original languageEnglish
Title of host publicationTechnical Proceedings of the 2008 NSTI Nanotechnology Conference and Trade Show, NSTI-Nanotech, Nanotechnology 2008
Pages662-665
Number of pages4
StatePublished - 2008
Externally publishedYes
Event2008 NSTI Nanotechnology Conference and Trade Show, NSTI Nanotech 2008 Joint Meeting, Nanotechnology 2008 - Quebec City, QC, United States
Duration: Jun 1 2008Jun 5 2008

Publication series

NameTechnical Proceedings of the 2008 NSTI Nanotechnology Conference and Trade Show, NSTI-Nanotech, Nanotechnology 2008
Volume3

Conference

Conference2008 NSTI Nanotechnology Conference and Trade Show, NSTI Nanotech 2008 Joint Meeting, Nanotechnology 2008
Country/TerritoryUnited States
CityQuebec City, QC
Period06/1/0806/5/08

Keywords

  • Discrete cosine transform
  • Numerical simulation
  • Patterned substrate
  • Spinodal decomposition

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