Nontrivial topology in the layered Dirac nodal-line semimetal candidate SrZnSb2 with distorted Sb square nets

Jinyu Liu, Pengfei Liu, Kyle Gordon, Eve Emmanouilidou, Jie Xing, David Graf, Bryan C. Chakoumakos, Yan Wu, Huibo Cao, Dan Dessau, Qihang Liu, Ni Ni

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Abstract

Dirac states hosted by Sb/Bi square nets are known to exist in the layered antiferromagnetic AMnX2 (A = CaSr/Ba/Eu/Yb, X=Sb/Bi) material family with the space group to be P4/nmm or I4/mmm. In this paper, we present a comprehensive study of quantum transport behaviors, angle-resolved photoemission spectroscopy (ARPES), and first-principles calculations on SrZnSb2, a nonmagnetic analog to AMnX2, which crystalizes in the pnma space group with distorted square nets. From the quantum oscillation measurements up to 35 T, three major frequencies including F1=103T, F2=127T, and F3=160T are identified. The effective masses of the quasiparticles associated with these frequencies are extracted, namely, m1∗=0.1 me, m2∗=0.1 me, and m3∗=0.09 me, where me is the free electron mass. From the three band Lifshitz-Kosevich fit, the Berry phases accumulated along the cyclotron orbit of the quasiparticles are 0.06π, 1.2π, and 0.74π for F1, F2, and F3, respectively. Combined with the ARPES data and the first-principles calculations, we reveal that F2 and F3 are associated with the two nontrivial Fermi pockets at the Brillouin zone edge while F1 is associated with the trivial Fermi pocket at the zone center. In addition, the first-principles calculations further suggest the existence of a Dirac nodal line in the band structure of SrZnSb2.

Original languageEnglish
Article number195123
JournalPhysical Review B
Volume100
Issue number19
DOIs
StatePublished - Nov 14 2019

Funding

Work at UCLA was supported by DOE Award DE-SC0011978. The National High Magnetic Field Laboratory is supported by the National Science Foundation through NSF/DMR-1644779 and the State of Florida. Work at ORNL was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, DOE. H.C. acknowledges the support from Office of Science, Office of Basic Energy Sciences, DOE under Award Number DE-AC05-00OR22725. P.L. and Q.L. acknowledge the support from the Guangdong Innovative and Entrepreneurial Research Team Program under Grant No. 2017ZT07C062 and Guangdong Provincial Key Laboratory for Computational Science and Material Design under Grant No. 2019B030301001. Work at the University of Colorado was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences under Award DE-FG02-03ER46066. The ARPES experiment used resources of the Advanced Light Source, which is a DOE Office of Science User Facility under Contract No. DE-AC02-05CH11231.

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