Neutron spin-echo investigation of slow spin dynamics in Kagomé-Bilayer frustrated magnets as evidence for phonon assisted relaxation in SrCr9xGa12-9xO19

H. Mutka, G. Ehlers, C. Payen, D. Bono, J. R. Stewart, P. Fouquet, P. Mendels, J. Y. Mevellec, N. Blanchard, G. Collin

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Abstract

A neutron spin-echo investigation of the low temperature spin dynamics in two well-characterized kagomé bilayer compounds SrCr9xGa12-9xO19 (x=0.95, SCGO) and Ba2Sn2ZnCr7xGa10-7xO22 (x=0.97, BSZCGO) reveals two novel features. One is the slowing down of the relaxation rate without critical behavior at Tg, where a macroscopic spin-glass-like freezing occurs. The second is, in SCGO at 4 K (∼ Tg)<T<7K, the relaxation rate activation energy Ea=7±0.4meV, equal to the energy of a phonon mode, pointing out the role of spin-lattice coupling.

Original languageEnglish
Article number047203
JournalPhysical Review Letters
Volume97
Issue number4
DOIs
StatePublished - 2006
Externally publishedYes

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