Neutron scattering studies of the spin-5/2 antiferromagnetic linear trimer substance SrMn3P4O14

  • Masashi Hase
  • , Andreas Dönni
  • , Kiyoshi Ozawa
  • , Hideaki Kitazawa
  • , Osamu Sakai
  • , Vladimir Yu Pomjakushin
  • , Lukas Keller
  • , Koji Kaneko
  • , Naoto Metoki
  • , Kazuhisa Kakurai
  • , Masaaki Matsuda
  • , Tao Yang
  • , Rihong Cong
  • , Jianhua Lin

    Research output: Contribution to journalConference articlepeer-review

    1 Scopus citations

    Abstract

    We studied the spin-5/2 antiferromagnetic (AF) linear trimer substance SrMn3P4O14 using neutron powder diffraction and inelastic neutron scattering (INS) techniques. We determined the magnetic structure below TN1 = 2.2(1) K. Ordered magnetic moments have x and z components. The angle between two neighboring moments in the trimer is 164 or 166° at 1.5 K, indicating that the intra-trimer (J1) interaction is AF as expected. The propagation vector is expressed as k = [0, ky, 0]. The value of ky is 0.317 at 1.5 K, indicating an incommensurate magnetic structure. The value of ky changes abruptly between 1.7 and 1.8 K and reaches values close to 0.33 above 1.8 K, indicating another phase transition at TN2 = 1.75(5) K. We observed plural magnetic excitations. The peak positions are 0.46, 0.68 and 1.02 meV. Our INS results are consistent with those expected in the trimer model. We evaluated the J 1 value as 0.29 meV (3.4 K).

    Original languageEnglish
    Article number012066
    JournalJournal of Physics: Conference Series
    Volume340
    DOIs
    StatePublished - 2012
    Event5th European Conference on Neutron Scattering, ECNS 2011 - Prague, Czech Republic
    Duration: Jul 17 2011Jul 21 2011

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