Neutron scattering and scaling behavior in URu2 Zn20 and YbFe2 Zn20

C. H. Wang, A. D. Christianson, J. M. Lawrence, E. D. Bauer, E. A. Goremychkin, A. I. Kolesnikov, F. Trouw, F. Ronning, J. D. Thompson, M. D. Lumsden, N. Ni, E. D. Mun, S. Jia, P. C. Canfield, Y. Qiu, J. R.D. Copley

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Abstract

The dynamic susceptibility χ⊃″ (ΔE), measured by inelastic neutron-scattering measurements, shows a broad peak centered at E max =15meV for the cubic actinide compound URu2 Zn 20 and 7 meV at zone center and at the (1/2, 1/2, 1/2) zone boundary for the rare-earth counterpart compound YbFe2 Zn20. For URu2 Zn20, the low-temperature susceptibility and magnetic specific-heat coefficient γ= Cmag /T take the values χ=0.011emu/mole and γ=190mJ/mole K2 at T=2K. These values are roughly three times smaller, and Emax is three times larger, than recently reported for the related compound UCo2 Zn20, so that χ and γ scale inversely with the characteristic energy for spin fluctuations, Tsf = Emax / kB. While χ (T), Cmag (T), and Emax of the 4f compound YbFe2 Zn20 are very well described by the Kondo impurity model, we show that the model works poorly for URu2 Zn20 and UCo 2 Zn20, suggesting that the scaling behavior of the actinide compounds arises from spin fluctuations of itinerant 5f electrons.

Original languageEnglish
Article number184407
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume82
Issue number18
DOIs
StatePublished - Nov 5 2010

Funding

FundersFunder number
Directorate for Mathematical and Physical Sciences0454672

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