Abstract
We study crystal field-phonon interactions in quantum spin liquid candidates C s Y b S e 2 with variable temperature, polarization, and magnetic-field dependent Raman microscopy. Complex interplay between phonon modes and CEF modes is observed in real space.
Original language | English |
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Title of host publication | 2022 Conference on Lasers and Electro-Optics, CLEO 2022 - Proceedings |
Publisher | Institute of Electrical and Electronics Engineers Inc. |
ISBN (Electronic) | 9781957171050 |
State | Published - 2022 |
Event | 2022 Conference on Lasers and Electro-Optics, CLEO 2022 - San Jose, United States Duration: May 15 2022 → May 20 2022 |
Publication series
Name | 2022 Conference on Lasers and Electro-Optics, CLEO 2022 - Proceedings |
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Conference
Conference | 2022 Conference on Lasers and Electro-Optics, CLEO 2022 |
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Country/Territory | United States |
City | San Jose |
Period | 05/15/22 → 05/20/22 |
Funding
This research was sponsored by the U. S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The first principles phonon calculations and Raman microscopy were performed at the Center for Nanophase Materials Sciences, which isaU.S. Department of Energy Office of Science User Facility. L.L. acknowledges computational resources ofthe Compute and Data Environment for Science (CADES) at the Oak Ridge National Laboratory, which is supported by the Office of Science ofthe U. S. Department of Energy under Contract No. DE-AC05-00OR22725. Postdoctoral research support was provided by the Intelligence Community Postdoctoral Research Fellowship Program at the Oak Ridge National Laboratory, administered by Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and the Office ofthe Director of National Intelligence.