Nanocellulose Dewatering and Drying: Current State and Future Perspectives

Scott Sinquefield, Peter N. Ciesielski, Kai Li, Douglas J. Gardner, Soydan Ozcan

Research output: Contribution to journalArticlepeer-review

105 Scopus citations

Abstract

The knowledge base for nanocellulose (NC) has grown exponentially over the past two decades and continues to expand with the increasing number of potential applications demonstrated in the literature and the patent space. NC has multiple forms depending on the starting cellulose source and the specific process used to produce it. Its high degree of surface reactivity makes it an ideal support structure for a wide variety of functional groups, leading to the ability to engineer materials for very specific applications. However, removing water from an NC suspension, e.g., dewatering and drying, while retaining the nanoscale properties of the NC remains a significant challenge to successful commercialization of NC materials. Processes for dewatering and drying of NC are desirable because of the high transport costs of shipping dilute aqueous suspensions, as well as end-use application requirements. Therefore, the development of nondestructive, cost-effective, scalable, and environmentally friendly dewatering and drying processes is important for commercial deployment of NC applications. This review addresses the current state of published knowledge on NC dewatering and drying and identifies research gaps that could be further explored in a precompetitive context to accelerate commercialization.

Original languageEnglish
Pages (from-to)9601-9615
Number of pages15
JournalACS Sustainable Chemistry and Engineering
Volume8
Issue number26
DOIs
StatePublished - Jul 6 2020

Funding

This manuscript has been authored in part by UT-Battelle, LLC, under Contract DE-AC05-00OR22725 with the U.S. Department of Energy (DOE). The U.S. government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan ( http://energy.gov/downloads/doe-public-access-plan) . We gratefully acknowledge the review comments and suggestions given by Dr. Kim Nelson of GranBio Co., by Dr. Robert Moon of the U.S. Forest Products Laboratory, and by Dr. Yousoo Han of the University of Maine. We gratefully acknowledge support and funding by the U.S. Endowment for Forestry & Communities, and by APPTI member companies. P.N.C. acknowledges support from the Office of Energy Efficiency and Renewable Energy, Bioenergy Technology Office of the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the Alliance for Sustainable Energy, LLC. K.L. and S.O. were supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office, under Contract DE-AC05-00OR22725 with UT-Battelle LLC.

FundersFunder number
APPTI
U.S. Department of Energy
Advanced Manufacturing OfficeDE-AC05-00OR22725
Office of Energy Efficiency and Renewable Energy
Bioenergy Technologies OfficeDE-AC36-08GO28308
U.S. Endowment for Forestry and Communities
UT-Battelle

    Keywords

    • Cellulose nanocrystals
    • Cellulose nanofibrils
    • Dewatering
    • Drying
    • Nanocellulose

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