Muon spin relaxation in the spin-ring system Cu3WO6: Quasistatic spin freezing at 7.0 K

Y. Fudamoto; I. M. Gat; M. I. Larkin; J. Merrin; B. Nachumi; A. T. Savici; Y. J. Uemura; G. M. Luke; K. M. Kojima; M. Hase; T. Masuda; K. Uchinokura

doi:10.1103/PhysRevB.65.174428

Muon spin relaxation in the spin-ring system Cu₃WO₆: Quasistatic spin freezing at 7.0 K

Y. Fudamoto
, I. M. Gat
, M. I. Larkin
, J. Merrin
, B. Nachumi
, A. T. Savici
, Y. J. Uemura
, G. M. Luke
, K. M. Kojima
, M. Hase
, T. Masuda
, K. Uchinokura

Research output: Contribution to journal › Article › peer-review

5 Scopus citations

Abstract

Quasistatic spin freezing is observed at T=7.0 K in the muon spin relaxation (μSR) measurements of polycrystalline Cu₃WO₆. This material has been widely considered to possess a nonmagnetic spin-singlet ground state based on the previous neutron scattering and susceptibility studies in which a spin gap was observed. Zn-doped Cu_3-xZn_xWO₆ with x>0, however, exhibit no signature of spin freezing. The μSR results of Cu_3-xZn_xWO₆ are similar to those of a charge-ordered system Na_xV₂O₅. A few interpretations of the observed spin freezing will be presented.

Original language	English
Article number	174428
Pages (from-to)	1744281-17442810
Number of pages	15698530
Journal	Physical Review B - Condensed Matter and Materials Physics
Volume	65
Issue number	17
DOIs	https://doi.org/10.1103/PhysRevB.65.174428
State	Published - May 1 2002
Externally published	Yes

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Fudamoto, Y., Gat, I. M., Larkin, M. I., Merrin, J., Nachumi, B., Savici, A. T., Uemura, Y. J., Luke, G. M., Kojima, K. M., Hase, M., Masuda, T., & Uchinokura, K. (2002). Muon spin relaxation in the spin-ring system Cu₃WO₆: Quasistatic spin freezing at 7.0 K. Physical Review B - Condensed Matter and Materials Physics, 65(17), 1744281-17442810. Article 174428. https://doi.org/10.1103/PhysRevB.65.174428

@article{47b6a73b5e68446e806377c86dcc44b6,

title = "Muon spin relaxation in the spin-ring system Cu3WO6: Quasistatic spin freezing at 7.0 K",

abstract = "Quasistatic spin freezing is observed at T=7.0 K in the muon spin relaxation (μSR) measurements of polycrystalline Cu3WO6. This material has been widely considered to possess a nonmagnetic spin-singlet ground state based on the previous neutron scattering and susceptibility studies in which a spin gap was observed. Zn-doped Cu3-xZnxWO6 with x>0, however, exhibit no signature of spin freezing. The μSR results of Cu3-xZnxWO6 are similar to those of a charge-ordered system NaxV2O5. A few interpretations of the observed spin freezing will be presented.",

author = "Y. Fudamoto and Gat, \{I. M.\} and Larkin, \{M. I.\} and J. Merrin and B. Nachumi and Savici, \{A. T.\} and Uemura, \{Y. J.\} and Luke, \{G. M.\} and Kojima, \{K. M.\} and M. Hase and T. Masuda and K. Uchinokura",

year = "2002",

month = may,

day = "1",

doi = "10.1103/PhysRevB.65.174428",

language = "English",

volume = "65",

pages = "1744281--17442810",

journal = "Physical Review B - Condensed Matter and Materials Physics",

issn = "0163-1829",

publisher = "American Physical Society",

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}

Fudamoto, Y, Gat, IM, Larkin, MI, Merrin, J, Nachumi, B, Savici, AT, Uemura, YJ, Luke, GM, Kojima, KM, Hase, M, Masuda, T & Uchinokura, K 2002, 'Muon spin relaxation in the spin-ring system Cu₃WO₆: Quasistatic spin freezing at 7.0 K', Physical Review B - Condensed Matter and Materials Physics, vol. 65, no. 17, 174428, pp. 1744281-17442810. https://doi.org/10.1103/PhysRevB.65.174428

TY - JOUR

T1 - Muon spin relaxation in the spin-ring system Cu3WO6

T2 - Quasistatic spin freezing at 7.0 K

AU - Fudamoto, Y.

AU - Gat, I. M.

AU - Larkin, M. I.

AU - Merrin, J.

AU - Nachumi, B.

AU - Savici, A. T.

AU - Uemura, Y. J.

AU - Luke, G. M.

AU - Kojima, K. M.

AU - Hase, M.

AU - Masuda, T.

AU - Uchinokura, K.

PY - 2002/5/1

Y1 - 2002/5/1

N2 - Quasistatic spin freezing is observed at T=7.0 K in the muon spin relaxation (μSR) measurements of polycrystalline Cu3WO6. This material has been widely considered to possess a nonmagnetic spin-singlet ground state based on the previous neutron scattering and susceptibility studies in which a spin gap was observed. Zn-doped Cu3-xZnxWO6 with x>0, however, exhibit no signature of spin freezing. The μSR results of Cu3-xZnxWO6 are similar to those of a charge-ordered system NaxV2O5. A few interpretations of the observed spin freezing will be presented.

AB - Quasistatic spin freezing is observed at T=7.0 K in the muon spin relaxation (μSR) measurements of polycrystalline Cu3WO6. This material has been widely considered to possess a nonmagnetic spin-singlet ground state based on the previous neutron scattering and susceptibility studies in which a spin gap was observed. Zn-doped Cu3-xZnxWO6 with x>0, however, exhibit no signature of spin freezing. The μSR results of Cu3-xZnxWO6 are similar to those of a charge-ordered system NaxV2O5. A few interpretations of the observed spin freezing will be presented.

UR - https://www.scopus.com/pages/publications/0036574988

U2 - 10.1103/PhysRevB.65.174428

DO - 10.1103/PhysRevB.65.174428

M3 - Article

AN - SCOPUS:0036574988

SN - 0163-1829

VL - 65

SP - 1744281

EP - 17442810

JO - Physical Review B - Condensed Matter and Materials Physics

JF - Physical Review B - Condensed Matter and Materials Physics

IS - 17

M1 - 174428

ER -

Muon spin relaxation in the spin-ring system Cu₃WO₆: Quasistatic spin freezing at 7.0 K

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