Abstract
Commonly produced as a byproduct of uranium fission, 99Mo is a key medical isotope that is in high demand in the United States. An international goal is to switch from medical isotope production technologies that require highly enriched uranium to medical isotope production technologies that require only low-enriched uranium. Niowave Inc. is contributing to this goal by developing an accelerator-driven subcritical assembly called the Uranium Target Assembly (UTA). This work compares the performance of Dakota’s Multi-Objective Genetic Algorithm (MOGA) against traditional sensitivity analysis in the neutronic optimization of the UTA-3 system. The design objectives are k-eigenvalue (keff) and natural uranium fission power, which are directly correlated with the amount of 99Mo produced. Dakota:MOGA did not perform as well as human engineering ingenuity in optimization studies with high numbers of input parameters, such as fuel rod type selection and fuel rod placement. However, Dakota:MOGA did outperform traditional sensitivity analysis in optimization studies with fewer than 20 parameters and revealed the degree to which each parameter influences the optimal design space for keff and natural uranium fission power (to a lesser extent). As the design model became more complex in the final stage of design, the computational resources required to calculate the design objective values in the Monte Carlo N-Particle transport code from selected input parameter combinations limited Dakota:MOGA’s performance, and, unfortunately, human intervention was required to discern the optimal design space. Future work will attempt to reduce computational resource constraints by incorporating areduced-order neutronics model into the optimization cycle.
| Original language | English |
|---|---|
| Journal | Nuclear Science and Engineering |
| DOIs | |
| State | Accepted/In press - 2025 |
Funding
The authors acknowledge the staff at Niowave Inc. for their support and collaboration throughout the design process. Financial support for this research was provided by the US Department of Energy’s (DOE’s) National Nuclear Security Administration Office of Material Management and Minimization’s Molybdenum-99 Program. The report was authored by UT-Battelle LLC under contract no. DE-AC05-00OR22725 with the DOE. The publisher acknowledges the US government license to provide public access under the DOE Public Access Plan ( http://energy.gov/downloads/doe-public-access-plan ). Notice: This manuscript has been authored by UT-Battelle LLC under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan ( https://www.energy.gov/doe-public-access-plan ).
Keywords
- Accelerator-driven systems
- genetic algorithm
- optimization
- photonuclear
- subcritical assembly