Measurements of liquid and glass structures using aerodynamic levitation and in-situ high energy x-ray and neutron scattering

J. K.R. Weber, C. J. Benmore, L. B. Skinner, J. Neuefeind, S. K. Tumber, G. Jennings, L. J. Santodonato, D. Jin, J. Du, J. B. Parise

Research output: Contribution to journalArticlepeer-review

43 Scopus citations

Abstract

Investigation of high temperature molten materials and their evolution to the amorphous state is often hampered by unwanted reactions with container surfaces. This work used aerodynamic levitation in combination with laser beam heating to study high melting point materials that can form supercooled liquids or glasses. Details of the instruments that are being used at the Advanced Photon Source and the Spallation Neutron Source to study molten oxides with high energy x-ray scattering and neutron diffraction with isotope substitution are presented. Examples of measurements are used to illustrate the use of the instruments. Plans for further development and application of the capabilities are presented.

Original languageEnglish
Pages (from-to)49-51
Number of pages3
JournalJournal of Non-Crystalline Solids
Volume383
DOIs
StatePublished - Jan 1 2014

Funding

Experimental design, sample synthesis and selection, data collection and analysis and preparation of the manuscript are supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contracts DE-FG02-09ER46650, DE-SC0004684, DE-SC0007564, and DE-AC02-06CH11357. We thank Bruce Hill and John Carruth at the Spallation Neutron Source and Rick Spence at the Advanced Photon Source for their help in setting up the levitator equipment.

Keywords

  • Glass
  • Levitation
  • Liquids
  • Neutron
  • X-ray

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