Abstract
The intermetallic UCu4+x Al8-xcompounds (0.1 ≤ x ≤ 1.95) have remarkable electronic and magnetic properties. The Cu-poor compositions within this x-range are antiferromagnetic (AF). The Néel temperature (TN) drops gradually from ∝ 36 K for x = 0.1 until AF is completely suppressed near x = 1.1, while the Sommerfeld coefficient (γ) increases dramatically with x, reaching a maximum value of 750mJ/molK2 for x = 1.75. Reported in this investigation are magnetoresistance (MR) and magnetic susceptibility (x) measurements at low temperatures (T) and high magnetic fields (B). The isothermal MR data below 40 K crosses over from positive in the low-x to negative in the high-x range. These results are interpreted in the context of spin fluctuations, hybridization, and non-magnetic atomic disorder.
| Original language | English |
|---|---|
| Pages (from-to) | 42-44 |
| Number of pages | 3 |
| Journal | Journal of Magnetism and Magnetic Materials |
| Volume | 226-230 |
| Issue number | PART I |
| DOIs | |
| State | Published - 2001 |
| Externally published | Yes |
Funding
The support of NSF Grant No. INT-9725929 (MST, AHL), FAPESP Grant No. 99/10798-0 (RFJ, RM), and CNPq (Brazil) (RFJ) are gratefully acknowledged. Work at the NHMFL was performed under the auspices of the NSF, the state of Florida, and the USDOE.
Keywords
- Antiferromagnetism
- Heavy fermions
- Magnetoresistance