Magnetic properties of the quasi-one-dimensional S=1 spin chain antiferromagnet BaNiTe2 O7

Xiyu Chen; Yiming Gao; Meifeng Liu; Tao Zou; V. Ovidiu Garlea; Clarina Dela Cruz; Zhen Liu; Wenjing Niu; Leili Tan; Guanzhong Zhou; Fei Liu; Shuhan Zheng; Zhen Ma; Xiuzhang Wang; Hong Li; Shuai Dong; Jun Ming Liu

doi:10.1103/PhysRevMaterials.7.094404

Magnetic properties of the quasi-one-dimensional S=1 spin chain antiferromagnet BaNiTe2 O7

Xiyu Chen, Yiming Gao, Meifeng Liu, Tao Zou, V. Ovidiu Garlea, Clarina Dela Cruz, Zhen Liu, Wenjing Niu, Leili Tan, Guanzhong Zhou, Fei Liu, Shuhan Zheng, Zhen Ma, Xiuzhang Wang, Hong Li, Shuai Dong, Jun Ming Liu

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Abstract

We report a quasi-one-dimensional S=1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a short-range magnetic correlation around T∼22K. With further cooling, an antiferromagnetic phase transition is observed at TN∼5.4K. Neutron powder diffraction revealed antiferromagnetic noncollinear order with a commensurate propagation vector k=(1/2,1,0). The refined magnetic moment size of Ni2+ at 1.5 K is 1.84μB, and its noncollinear spin texture is confirmed by first-principles calculations. Inelastic neutron-scattering results and density functional theory calculations confirmed the quasi-one-dimensional nature of the spin systems.

Original language	English
Article number	094404
Journal	Physical Review Materials
Volume	7
Issue number	9
DOIs	https://doi.org/10.1103/PhysRevMaterials.7.094404
State	Published - Sep 2023

Funding

This work was supported by the National Natural Science Foundation of China (Grants No. 12074111, No. 52272108, No. 92163210, and No. 11834002). National Natural Science Foundation of China No. 12204160 and the Hubei Provincial Natural Science Foundation of China with Grant No. 2023AFA105. A portion of this research used resources at High Flux Isotope Reactor and Spallation Neutron Source, DOE Office of Science User Facilities operated by the Oak Ridge National Laboratory. Y.M.G. and S.D. thank the Big Data Center of Southeast University for providing the facility support for the calculations.

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Chen, X., Gao, Y., Liu, M., Zou, T., Garlea, V. O., Dela Cruz, C., Liu, Z., Niu, W., Tan, L., Zhou, G., Liu, F., Zheng, S., Ma, Z., Wang, X., Li, H., Dong, S., & Liu, J. M. (2023). Magnetic properties of the quasi-one-dimensional S=1 spin chain antiferromagnet BaNiTe2 O7. Physical Review Materials, 7(9), Article 094404. https://doi.org/10.1103/PhysRevMaterials.7.094404

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title = "Magnetic properties of the quasi-one-dimensional S=1 spin chain antiferromagnet BaNiTe2 O7",

abstract = "We report a quasi-one-dimensional S=1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a short-range magnetic correlation around T∼22K. With further cooling, an antiferromagnetic phase transition is observed at TN∼5.4K. Neutron powder diffraction revealed antiferromagnetic noncollinear order with a commensurate propagation vector k=(1/2,1,0). The refined magnetic moment size of Ni2+ at 1.5 K is 1.84μB, and its noncollinear spin texture is confirmed by first-principles calculations. Inelastic neutron-scattering results and density functional theory calculations confirmed the quasi-one-dimensional nature of the spin systems.",

author = "Xiyu Chen and Yiming Gao and Meifeng Liu and Tao Zou and Garlea, {V. Ovidiu} and {Dela Cruz}, Clarina and Zhen Liu and Wenjing Niu and Leili Tan and Guanzhong Zhou and Fei Liu and Shuhan Zheng and Zhen Ma and Xiuzhang Wang and Hong Li and Shuai Dong and Liu, {Jun Ming}",

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year = "2023",

month = sep,

doi = "10.1103/PhysRevMaterials.7.094404",

language = "English",

volume = "7",

journal = "Physical Review Materials",

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T1 - Magnetic properties of the quasi-one-dimensional S=1 spin chain antiferromagnet BaNiTe2 O7

AU - Chen, Xiyu

AU - Gao, Yiming

AU - Liu, Meifeng

AU - Zou, Tao

AU - Garlea, V. Ovidiu

AU - Dela Cruz, Clarina

AU - Liu, Zhen

AU - Niu, Wenjing

AU - Tan, Leili

AU - Zhou, Guanzhong

AU - Liu, Fei

AU - Zheng, Shuhan

AU - Ma, Zhen

AU - Wang, Xiuzhang

AU - Li, Hong

AU - Dong, Shuai

AU - Liu, Jun Ming

PY - 2023/9

Y1 - 2023/9

N2 - We report a quasi-one-dimensional S=1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a short-range magnetic correlation around T∼22K. With further cooling, an antiferromagnetic phase transition is observed at TN∼5.4K. Neutron powder diffraction revealed antiferromagnetic noncollinear order with a commensurate propagation vector k=(1/2,1,0). The refined magnetic moment size of Ni2+ at 1.5 K is 1.84μB, and its noncollinear spin texture is confirmed by first-principles calculations. Inelastic neutron-scattering results and density functional theory calculations confirmed the quasi-one-dimensional nature of the spin systems.

AB - We report a quasi-one-dimensional S=1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a short-range magnetic correlation around T∼22K. With further cooling, an antiferromagnetic phase transition is observed at TN∼5.4K. Neutron powder diffraction revealed antiferromagnetic noncollinear order with a commensurate propagation vector k=(1/2,1,0). The refined magnetic moment size of Ni2+ at 1.5 K is 1.84μB, and its noncollinear spin texture is confirmed by first-principles calculations. Inelastic neutron-scattering results and density functional theory calculations confirmed the quasi-one-dimensional nature of the spin systems.

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VL - 7

JO - Physical Review Materials

JF - Physical Review Materials

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M1 - 094404

ER -

Magnetic properties of the quasi-one-dimensional S=1 spin chain antiferromagnet BaNiTe2 O7

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