Low-energy spin dynamics of orthoferrites AFeO3 (A = Y, La, Bi)

Kisoo Park, Hasung Sim, Jonathan C. Leiner, Yoshiyuki Yoshida, Jaehong Jeong, Shin Ichiro Yano, Jason Gardner, Philippe Bourges, Milan Klicpera, Vladimír Sechovský, Martin Boehm, Je Geun Park

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24 Scopus citations

Abstract

YFeO3 and LaFeO3 are members of the rare-earth orthoferrites family with Pbnm space group. Using inelastic neutron scattering, the low-energy spin excitations have been measured around the magnetic Brillouin zone center. Splitting of magnon branches and finite magnon gaps (∼2 meV) are observed for both compounds, where the Dzyaloshinsky-Moriya interactions account for most of this gap with some additional contribution from single-ion anisotropy. We also make comparisons with multiferroic BiFeO3 (R3c space group), in which similar behavior was observed. By taking into account all relevant local Dzyaloshinsky-Moriya interactions, our analysis allows for the precise determination of all experimentally observed parameters in the spin-Hamiltonian. We find that different properties of the Pbnm and R3c space group lead to the stabilization of a spin cycloid structure in the latter case but not in the former, which explains the difference in the levels of complexity of magnon band structures for the respective compounds.

Original languageEnglish
Article number235802
JournalJournal of Physics Condensed Matter
Volume30
Issue number23
DOIs
StatePublished - May 14 2018
Externally publishedYes

Funding

We thank Joosung Oh, Y Noda and D T Adroja for fruitful discussions. This work was supported by the Institute of Basic Science in Korea (Grant No. IBS-R009-G1). The work of MK and VS was supported within the program of Large Infrastructures for Research, Experimental Development and Innovation (project No. LM2015050) and project LTT17019 financed by the Ministry of Education, Youth and Sports, Czech Republic.

FundersFunder number
Ministry of Education, Youth and Sports, Czech Republic

    Keywords

    • DzyaloshinskiiMoriya interaction
    • ferrites
    • inelastic neutron scattering
    • multiferroics
    • weak ferromagnetism

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